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Topological Defects Created by Gamma Rays in a Carbon Nanotube Bilayer

Graphene sheets are a highly radiation-resistant material for prospective nuclear applications and nanoscale defect engineering. However, the precise mechanism of graphene radiation hardness has remained elusive. In this paper, we study the origin and nature of defects induced by gamma radiation in...

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Autores principales: Grushevskaya, Halina, Timoshchenko, Andrey, Lipnevich, Ihor
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9921100/
https://www.ncbi.nlm.nih.gov/pubmed/36770369
http://dx.doi.org/10.3390/nano13030410
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author Grushevskaya, Halina
Timoshchenko, Andrey
Lipnevich, Ihor
author_facet Grushevskaya, Halina
Timoshchenko, Andrey
Lipnevich, Ihor
author_sort Grushevskaya, Halina
collection PubMed
description Graphene sheets are a highly radiation-resistant material for prospective nuclear applications and nanoscale defect engineering. However, the precise mechanism of graphene radiation hardness has remained elusive. In this paper, we study the origin and nature of defects induced by gamma radiation in a graphene rolled-up plane. In order to reduce the environmental influence on graphene and reveal the small effects of gamma rays, we have synthesized a novel graphene-based nanocomposite material containing a bilayer of highly aligned carbon nanotube assemblies that have been decorated by organometallic compounds and suspended on nanoporous Al [Formula: see text] O [Formula: see text] membranes. The bilayer samples were irradiated by gamma rays from a [Formula: see text] Cs source with a fluence rate of the order of [Formula: see text] m [Formula: see text] s [Formula: see text]. The interaction between the samples and gamma quanta results in the appearance of three characteristic photon escape peaks in the radiation spectra. We explain the mechanism of interaction between the graphene sheets and gamma radiation using a pseudo-Majorana fermion graphene model, which is a quasi-relativistic [Formula: see text]-flavor graphene model with a Majorana-like mass term. This model admits the existence of giant charge carrier currents that are sufficient to neutralize the impact of ionizing radiation. Experimental evidence is provided for the prediction that the 661.7-keV gamma quanta transfer enough energy to the electron subsystem of graphene to bring about the deconfinement of the bound pseudo-Majorana modes and involve C atoms in a vortical motion of the electron density flows in the graphene plane. We explain the radiation hardness of graphene by the topological non-triviality of the pseudo-Majorana fermion configurations comprising the graphene charge carriers.
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spelling pubmed-99211002023-02-12 Topological Defects Created by Gamma Rays in a Carbon Nanotube Bilayer Grushevskaya, Halina Timoshchenko, Andrey Lipnevich, Ihor Nanomaterials (Basel) Article Graphene sheets are a highly radiation-resistant material for prospective nuclear applications and nanoscale defect engineering. However, the precise mechanism of graphene radiation hardness has remained elusive. In this paper, we study the origin and nature of defects induced by gamma radiation in a graphene rolled-up plane. In order to reduce the environmental influence on graphene and reveal the small effects of gamma rays, we have synthesized a novel graphene-based nanocomposite material containing a bilayer of highly aligned carbon nanotube assemblies that have been decorated by organometallic compounds and suspended on nanoporous Al [Formula: see text] O [Formula: see text] membranes. The bilayer samples were irradiated by gamma rays from a [Formula: see text] Cs source with a fluence rate of the order of [Formula: see text] m [Formula: see text] s [Formula: see text]. The interaction between the samples and gamma quanta results in the appearance of three characteristic photon escape peaks in the radiation spectra. We explain the mechanism of interaction between the graphene sheets and gamma radiation using a pseudo-Majorana fermion graphene model, which is a quasi-relativistic [Formula: see text]-flavor graphene model with a Majorana-like mass term. This model admits the existence of giant charge carrier currents that are sufficient to neutralize the impact of ionizing radiation. Experimental evidence is provided for the prediction that the 661.7-keV gamma quanta transfer enough energy to the electron subsystem of graphene to bring about the deconfinement of the bound pseudo-Majorana modes and involve C atoms in a vortical motion of the electron density flows in the graphene plane. We explain the radiation hardness of graphene by the topological non-triviality of the pseudo-Majorana fermion configurations comprising the graphene charge carriers. MDPI 2023-01-19 /pmc/articles/PMC9921100/ /pubmed/36770369 http://dx.doi.org/10.3390/nano13030410 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Grushevskaya, Halina
Timoshchenko, Andrey
Lipnevich, Ihor
Topological Defects Created by Gamma Rays in a Carbon Nanotube Bilayer
title Topological Defects Created by Gamma Rays in a Carbon Nanotube Bilayer
title_full Topological Defects Created by Gamma Rays in a Carbon Nanotube Bilayer
title_fullStr Topological Defects Created by Gamma Rays in a Carbon Nanotube Bilayer
title_full_unstemmed Topological Defects Created by Gamma Rays in a Carbon Nanotube Bilayer
title_short Topological Defects Created by Gamma Rays in a Carbon Nanotube Bilayer
title_sort topological defects created by gamma rays in a carbon nanotube bilayer
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9921100/
https://www.ncbi.nlm.nih.gov/pubmed/36770369
http://dx.doi.org/10.3390/nano13030410
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