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Quasi-BIC Modes in All-Dielectric Slotted Nanoantennas for Enhanced Er(3+) Emission

[Image: see text] In the quest for new and increasingly efficient photon sources, the engineering of the photonic environment at the subwavelength scale is fundamental for controlling the properties of quantum emitters. A high refractive index particle can be exploited to enhance the optical propert...

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Detalles Bibliográficos
Autores principales: Kalinic, Boris, Cesca, Tiziana, Balasa, Ionut Gabriel, Trevisani, Mirko, Jacassi, Andrea, Maier, Stefan A., Sapienza, Riccardo, Mattei, Giovanni
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9936627/
https://www.ncbi.nlm.nih.gov/pubmed/36820324
http://dx.doi.org/10.1021/acsphotonics.2c01703
Descripción
Sumario:[Image: see text] In the quest for new and increasingly efficient photon sources, the engineering of the photonic environment at the subwavelength scale is fundamental for controlling the properties of quantum emitters. A high refractive index particle can be exploited to enhance the optical properties of nearby emitters without decreasing their quantum efficiency, but the relatively modest Q-factors (Q ∼ 5–10) limit the local density of optical states (LDOS) amplification achievable. On the other hand, ultrahigh Q-factors (up to Q ∼ 10(9)) have been reported for quasi-BIC modes in all-dielectric nanostructures. In the present work, we demonstrate that the combination of quasi-BIC modes with high spectral confinement and nanogaps with spacial confinement in silicon slotted nanoantennas lead to a significant boosting of the electromagnetic LDOS in the optically active region of the nanoantenna array. We observe an enhancement of up to 3 orders of magnitude in the photoluminescence intensity and 2 orders of magnitude in the decay rate of the Er(3+) emission at room temperature and telecom wavelengths. Moreover, the nanoantenna directivity is increased, proving that strong beaming effects can be obtained when the emitted radiation couples to the high Q-factor modes. Finally, via tuning the nanoanntenna aspect ratio, a selective control of the Er(3+) electric and magnetic radiative transitions can be obtained, keeping the quantum efficiency almost unitary.