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Quasi-BIC Modes in All-Dielectric Slotted Nanoantennas for Enhanced Er(3+) Emission

[Image: see text] In the quest for new and increasingly efficient photon sources, the engineering of the photonic environment at the subwavelength scale is fundamental for controlling the properties of quantum emitters. A high refractive index particle can be exploited to enhance the optical propert...

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Autores principales: Kalinic, Boris, Cesca, Tiziana, Balasa, Ionut Gabriel, Trevisani, Mirko, Jacassi, Andrea, Maier, Stefan A., Sapienza, Riccardo, Mattei, Giovanni
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9936627/
https://www.ncbi.nlm.nih.gov/pubmed/36820324
http://dx.doi.org/10.1021/acsphotonics.2c01703
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author Kalinic, Boris
Cesca, Tiziana
Balasa, Ionut Gabriel
Trevisani, Mirko
Jacassi, Andrea
Maier, Stefan A.
Sapienza, Riccardo
Mattei, Giovanni
author_facet Kalinic, Boris
Cesca, Tiziana
Balasa, Ionut Gabriel
Trevisani, Mirko
Jacassi, Andrea
Maier, Stefan A.
Sapienza, Riccardo
Mattei, Giovanni
author_sort Kalinic, Boris
collection PubMed
description [Image: see text] In the quest for new and increasingly efficient photon sources, the engineering of the photonic environment at the subwavelength scale is fundamental for controlling the properties of quantum emitters. A high refractive index particle can be exploited to enhance the optical properties of nearby emitters without decreasing their quantum efficiency, but the relatively modest Q-factors (Q ∼ 5–10) limit the local density of optical states (LDOS) amplification achievable. On the other hand, ultrahigh Q-factors (up to Q ∼ 10(9)) have been reported for quasi-BIC modes in all-dielectric nanostructures. In the present work, we demonstrate that the combination of quasi-BIC modes with high spectral confinement and nanogaps with spacial confinement in silicon slotted nanoantennas lead to a significant boosting of the electromagnetic LDOS in the optically active region of the nanoantenna array. We observe an enhancement of up to 3 orders of magnitude in the photoluminescence intensity and 2 orders of magnitude in the decay rate of the Er(3+) emission at room temperature and telecom wavelengths. Moreover, the nanoantenna directivity is increased, proving that strong beaming effects can be obtained when the emitted radiation couples to the high Q-factor modes. Finally, via tuning the nanoanntenna aspect ratio, a selective control of the Er(3+) electric and magnetic radiative transitions can be obtained, keeping the quantum efficiency almost unitary.
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spelling pubmed-99366272023-02-18 Quasi-BIC Modes in All-Dielectric Slotted Nanoantennas for Enhanced Er(3+) Emission Kalinic, Boris Cesca, Tiziana Balasa, Ionut Gabriel Trevisani, Mirko Jacassi, Andrea Maier, Stefan A. Sapienza, Riccardo Mattei, Giovanni ACS Photonics [Image: see text] In the quest for new and increasingly efficient photon sources, the engineering of the photonic environment at the subwavelength scale is fundamental for controlling the properties of quantum emitters. A high refractive index particle can be exploited to enhance the optical properties of nearby emitters without decreasing their quantum efficiency, but the relatively modest Q-factors (Q ∼ 5–10) limit the local density of optical states (LDOS) amplification achievable. On the other hand, ultrahigh Q-factors (up to Q ∼ 10(9)) have been reported for quasi-BIC modes in all-dielectric nanostructures. In the present work, we demonstrate that the combination of quasi-BIC modes with high spectral confinement and nanogaps with spacial confinement in silicon slotted nanoantennas lead to a significant boosting of the electromagnetic LDOS in the optically active region of the nanoantenna array. We observe an enhancement of up to 3 orders of magnitude in the photoluminescence intensity and 2 orders of magnitude in the decay rate of the Er(3+) emission at room temperature and telecom wavelengths. Moreover, the nanoantenna directivity is increased, proving that strong beaming effects can be obtained when the emitted radiation couples to the high Q-factor modes. Finally, via tuning the nanoanntenna aspect ratio, a selective control of the Er(3+) electric and magnetic radiative transitions can be obtained, keeping the quantum efficiency almost unitary. American Chemical Society 2023-01-18 /pmc/articles/PMC9936627/ /pubmed/36820324 http://dx.doi.org/10.1021/acsphotonics.2c01703 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Kalinic, Boris
Cesca, Tiziana
Balasa, Ionut Gabriel
Trevisani, Mirko
Jacassi, Andrea
Maier, Stefan A.
Sapienza, Riccardo
Mattei, Giovanni
Quasi-BIC Modes in All-Dielectric Slotted Nanoantennas for Enhanced Er(3+) Emission
title Quasi-BIC Modes in All-Dielectric Slotted Nanoantennas for Enhanced Er(3+) Emission
title_full Quasi-BIC Modes in All-Dielectric Slotted Nanoantennas for Enhanced Er(3+) Emission
title_fullStr Quasi-BIC Modes in All-Dielectric Slotted Nanoantennas for Enhanced Er(3+) Emission
title_full_unstemmed Quasi-BIC Modes in All-Dielectric Slotted Nanoantennas for Enhanced Er(3+) Emission
title_short Quasi-BIC Modes in All-Dielectric Slotted Nanoantennas for Enhanced Er(3+) Emission
title_sort quasi-bic modes in all-dielectric slotted nanoantennas for enhanced er(3+) emission
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9936627/
https://www.ncbi.nlm.nih.gov/pubmed/36820324
http://dx.doi.org/10.1021/acsphotonics.2c01703
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