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Quantum Control by Few-Cycles Pulses: The Two-Level Problem

We investigate the problem of population transfer in a two-states system driven by an external electromagnetic field featuring a few cycles, until the extreme limit of two or one cycle. Taking the physical constraint of zero-area total field into account, we determine strategies leading to ultrahigh...

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Detalles Bibliográficos
Autores principales: Peyraut, François, Holweck, Frédéric, Guérin, Stéphane
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9955166/
https://www.ncbi.nlm.nih.gov/pubmed/36832579
http://dx.doi.org/10.3390/e25020212
Descripción
Sumario:We investigate the problem of population transfer in a two-states system driven by an external electromagnetic field featuring a few cycles, until the extreme limit of two or one cycle. Taking the physical constraint of zero-area total field into account, we determine strategies leading to ultrahigh-fidelity population transfer despite the failure of the rotating wave approximation. We specifically implement adiabatic passage based on adiabatic Floquet theory for a number of cycles as low as 2.5 cycles, finding and making the dynamics follow an adiabatic trajectory connecting the initial and targeted states. Nonadiabatic strategies with shaped or chirped pulses, extending the [Formula: see text]-pulse regime to two- or single-cycle pulses, are also derived.