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Complex-tensor theory of simple smectics
Matter self-assembling into layers generates unique properties, including structures of stacked surfaces, directed transport, and compact area maximization that can be highly functionalized in biology and technology. Smectics represent the paradigm of such lamellar materials — they are a state betwe...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9958025/ https://www.ncbi.nlm.nih.gov/pubmed/36828813 http://dx.doi.org/10.1038/s41467-023-36506-z |
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author | Paget, Jack Mazza, Marco G. Archer, Andrew J. Shendruk, Tyler N. |
author_facet | Paget, Jack Mazza, Marco G. Archer, Andrew J. Shendruk, Tyler N. |
author_sort | Paget, Jack |
collection | PubMed |
description | Matter self-assembling into layers generates unique properties, including structures of stacked surfaces, directed transport, and compact area maximization that can be highly functionalized in biology and technology. Smectics represent the paradigm of such lamellar materials — they are a state between fluids and solids, characterized by both orientational and partial positional ordering in one layering direction, making them notoriously difficult to model, particularly in confining geometries. We propose a complex tensor order parameter to describe the local degree of lamellar ordering, layer displacement and orientation of the layers for simple, lamellar smectics. The theory accounts for both dislocations and disclinations, by regularizing singularities within defect cores and so remaining continuous everywhere. The ability to describe disclinations and dislocation allows this theory to simulate arrested configurations and inclusion-induced local ordering. This tensorial theory for simple smectics considerably simplifies numerics, facilitating studies on the mesoscopic structure of topologically complex systems. |
format | Online Article Text |
id | pubmed-9958025 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-99580252023-02-26 Complex-tensor theory of simple smectics Paget, Jack Mazza, Marco G. Archer, Andrew J. Shendruk, Tyler N. Nat Commun Article Matter self-assembling into layers generates unique properties, including structures of stacked surfaces, directed transport, and compact area maximization that can be highly functionalized in biology and technology. Smectics represent the paradigm of such lamellar materials — they are a state between fluids and solids, characterized by both orientational and partial positional ordering in one layering direction, making them notoriously difficult to model, particularly in confining geometries. We propose a complex tensor order parameter to describe the local degree of lamellar ordering, layer displacement and orientation of the layers for simple, lamellar smectics. The theory accounts for both dislocations and disclinations, by regularizing singularities within defect cores and so remaining continuous everywhere. The ability to describe disclinations and dislocation allows this theory to simulate arrested configurations and inclusion-induced local ordering. This tensorial theory for simple smectics considerably simplifies numerics, facilitating studies on the mesoscopic structure of topologically complex systems. Nature Publishing Group UK 2023-02-24 /pmc/articles/PMC9958025/ /pubmed/36828813 http://dx.doi.org/10.1038/s41467-023-36506-z Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Paget, Jack Mazza, Marco G. Archer, Andrew J. Shendruk, Tyler N. Complex-tensor theory of simple smectics |
title | Complex-tensor theory of simple smectics |
title_full | Complex-tensor theory of simple smectics |
title_fullStr | Complex-tensor theory of simple smectics |
title_full_unstemmed | Complex-tensor theory of simple smectics |
title_short | Complex-tensor theory of simple smectics |
title_sort | complex-tensor theory of simple smectics |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9958025/ https://www.ncbi.nlm.nih.gov/pubmed/36828813 http://dx.doi.org/10.1038/s41467-023-36506-z |
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