Cargando…

High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface

Among the transitional metal dichalcogenides (TMDCs), molybdenum disulfide (MoS(2)) is considered an outstanding candidate for biosensing applications due to its high absorptivity and amenability to ionic current measurements. Dielectric metasurfaces have also emerged as a powerful platform for nove...

Descripción completa

Detalles Bibliográficos
Autores principales: Hajian, Hodjat, Rukhlenko, Ivan D., Bradley, A. Louise, Ozbay, Ekmel
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9959146/
https://www.ncbi.nlm.nih.gov/pubmed/36838070
http://dx.doi.org/10.3390/mi14020370
_version_ 1784895201800617984
author Hajian, Hodjat
Rukhlenko, Ivan D.
Bradley, A. Louise
Ozbay, Ekmel
author_facet Hajian, Hodjat
Rukhlenko, Ivan D.
Bradley, A. Louise
Ozbay, Ekmel
author_sort Hajian, Hodjat
collection PubMed
description Among the transitional metal dichalcogenides (TMDCs), molybdenum disulfide (MoS(2)) is considered an outstanding candidate for biosensing applications due to its high absorptivity and amenability to ionic current measurements. Dielectric metasurfaces have also emerged as a powerful platform for novel optical biosensing due to their low optical losses and strong near-field enhancements. Once functionalized with TMDCs, dielectric metasurfaces can also provide strong photon–exciton interactions. Here, we theoretically integrated a single layer of MoS(2) into a CMOS-compatible asymmetric dielectric metasurface composed of TiO(2) meta-atoms with a broken in-plane inversion symmetry on an SiO(2) substrate. We numerically show that the designed MoS(2)-integrated metasurface can function as a high-figure-of-merit ([Formula: see text]) van der Waals-based biosensor due to the support of quasi-bound states in the continuum. Moreover, owing to the critical coupling of the magnetic dipole resonances of the metasurface and the A exciton of the single layer of MoS(2), one can achieve a [Formula: see text] enhanced excitonic absorption by this two-port system. Therefore, the proposed design can function as an effective biosensor and is also practical for enhanced excitonic absorption and emission applications.
format Online
Article
Text
id pubmed-9959146
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher MDPI
record_format MEDLINE/PubMed
spelling pubmed-99591462023-02-26 High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface Hajian, Hodjat Rukhlenko, Ivan D. Bradley, A. Louise Ozbay, Ekmel Micromachines (Basel) Article Among the transitional metal dichalcogenides (TMDCs), molybdenum disulfide (MoS(2)) is considered an outstanding candidate for biosensing applications due to its high absorptivity and amenability to ionic current measurements. Dielectric metasurfaces have also emerged as a powerful platform for novel optical biosensing due to their low optical losses and strong near-field enhancements. Once functionalized with TMDCs, dielectric metasurfaces can also provide strong photon–exciton interactions. Here, we theoretically integrated a single layer of MoS(2) into a CMOS-compatible asymmetric dielectric metasurface composed of TiO(2) meta-atoms with a broken in-plane inversion symmetry on an SiO(2) substrate. We numerically show that the designed MoS(2)-integrated metasurface can function as a high-figure-of-merit ([Formula: see text]) van der Waals-based biosensor due to the support of quasi-bound states in the continuum. Moreover, owing to the critical coupling of the magnetic dipole resonances of the metasurface and the A exciton of the single layer of MoS(2), one can achieve a [Formula: see text] enhanced excitonic absorption by this two-port system. Therefore, the proposed design can function as an effective biosensor and is also practical for enhanced excitonic absorption and emission applications. MDPI 2023-02-01 /pmc/articles/PMC9959146/ /pubmed/36838070 http://dx.doi.org/10.3390/mi14020370 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Hajian, Hodjat
Rukhlenko, Ivan D.
Bradley, A. Louise
Ozbay, Ekmel
High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface
title High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface
title_full High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface
title_fullStr High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface
title_full_unstemmed High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface
title_short High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface
title_sort high-figure-of-merit biosensing and enhanced excitonic absorption in an mos(2)-integrated dielectric metasurface
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9959146/
https://www.ncbi.nlm.nih.gov/pubmed/36838070
http://dx.doi.org/10.3390/mi14020370
work_keys_str_mv AT hajianhodjat highfigureofmeritbiosensingandenhancedexcitonicabsorptioninanmos2integrateddielectricmetasurface
AT rukhlenkoivand highfigureofmeritbiosensingandenhancedexcitonicabsorptioninanmos2integrateddielectricmetasurface
AT bradleyalouise highfigureofmeritbiosensingandenhancedexcitonicabsorptioninanmos2integrateddielectricmetasurface
AT ozbayekmel highfigureofmeritbiosensingandenhancedexcitonicabsorptioninanmos2integrateddielectricmetasurface