Cargando…
High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface
Among the transitional metal dichalcogenides (TMDCs), molybdenum disulfide (MoS(2)) is considered an outstanding candidate for biosensing applications due to its high absorptivity and amenability to ionic current measurements. Dielectric metasurfaces have also emerged as a powerful platform for nove...
Autores principales: | , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2023
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9959146/ https://www.ncbi.nlm.nih.gov/pubmed/36838070 http://dx.doi.org/10.3390/mi14020370 |
_version_ | 1784895201800617984 |
---|---|
author | Hajian, Hodjat Rukhlenko, Ivan D. Bradley, A. Louise Ozbay, Ekmel |
author_facet | Hajian, Hodjat Rukhlenko, Ivan D. Bradley, A. Louise Ozbay, Ekmel |
author_sort | Hajian, Hodjat |
collection | PubMed |
description | Among the transitional metal dichalcogenides (TMDCs), molybdenum disulfide (MoS(2)) is considered an outstanding candidate for biosensing applications due to its high absorptivity and amenability to ionic current measurements. Dielectric metasurfaces have also emerged as a powerful platform for novel optical biosensing due to their low optical losses and strong near-field enhancements. Once functionalized with TMDCs, dielectric metasurfaces can also provide strong photon–exciton interactions. Here, we theoretically integrated a single layer of MoS(2) into a CMOS-compatible asymmetric dielectric metasurface composed of TiO(2) meta-atoms with a broken in-plane inversion symmetry on an SiO(2) substrate. We numerically show that the designed MoS(2)-integrated metasurface can function as a high-figure-of-merit ([Formula: see text]) van der Waals-based biosensor due to the support of quasi-bound states in the continuum. Moreover, owing to the critical coupling of the magnetic dipole resonances of the metasurface and the A exciton of the single layer of MoS(2), one can achieve a [Formula: see text] enhanced excitonic absorption by this two-port system. Therefore, the proposed design can function as an effective biosensor and is also practical for enhanced excitonic absorption and emission applications. |
format | Online Article Text |
id | pubmed-9959146 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-99591462023-02-26 High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface Hajian, Hodjat Rukhlenko, Ivan D. Bradley, A. Louise Ozbay, Ekmel Micromachines (Basel) Article Among the transitional metal dichalcogenides (TMDCs), molybdenum disulfide (MoS(2)) is considered an outstanding candidate for biosensing applications due to its high absorptivity and amenability to ionic current measurements. Dielectric metasurfaces have also emerged as a powerful platform for novel optical biosensing due to their low optical losses and strong near-field enhancements. Once functionalized with TMDCs, dielectric metasurfaces can also provide strong photon–exciton interactions. Here, we theoretically integrated a single layer of MoS(2) into a CMOS-compatible asymmetric dielectric metasurface composed of TiO(2) meta-atoms with a broken in-plane inversion symmetry on an SiO(2) substrate. We numerically show that the designed MoS(2)-integrated metasurface can function as a high-figure-of-merit ([Formula: see text]) van der Waals-based biosensor due to the support of quasi-bound states in the continuum. Moreover, owing to the critical coupling of the magnetic dipole resonances of the metasurface and the A exciton of the single layer of MoS(2), one can achieve a [Formula: see text] enhanced excitonic absorption by this two-port system. Therefore, the proposed design can function as an effective biosensor and is also practical for enhanced excitonic absorption and emission applications. MDPI 2023-02-01 /pmc/articles/PMC9959146/ /pubmed/36838070 http://dx.doi.org/10.3390/mi14020370 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Hajian, Hodjat Rukhlenko, Ivan D. Bradley, A. Louise Ozbay, Ekmel High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface |
title | High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface |
title_full | High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface |
title_fullStr | High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface |
title_full_unstemmed | High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface |
title_short | High-Figure-of-Merit Biosensing and Enhanced Excitonic Absorption in an MoS(2)-Integrated Dielectric Metasurface |
title_sort | high-figure-of-merit biosensing and enhanced excitonic absorption in an mos(2)-integrated dielectric metasurface |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9959146/ https://www.ncbi.nlm.nih.gov/pubmed/36838070 http://dx.doi.org/10.3390/mi14020370 |
work_keys_str_mv | AT hajianhodjat highfigureofmeritbiosensingandenhancedexcitonicabsorptioninanmos2integrateddielectricmetasurface AT rukhlenkoivand highfigureofmeritbiosensingandenhancedexcitonicabsorptioninanmos2integrateddielectricmetasurface AT bradleyalouise highfigureofmeritbiosensingandenhancedexcitonicabsorptioninanmos2integrateddielectricmetasurface AT ozbayekmel highfigureofmeritbiosensingandenhancedexcitonicabsorptioninanmos2integrateddielectricmetasurface |