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Highly Dispersed Pt-Incorporated Mesoporous Fe(2)O(3) for Low-Level Sensing of Formaldehyde Gas

Highly dispersed Pt-incorporated mesoporous Fe(2)O(3) (Pt/m-Fe(2)O(3)) of 4 μm size is prepared through a simple hydrothermal reaction and thermal decomposition procedures. Furthermore, the formaldehyde gas-sensing properties of Pt/m-Fe(2)O(3) are investigated. Compared with our previous mesoporous...

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Autores principales: Jeon, Seung Jin, Oh, Kyung Hee, Choi, Youngbo, Park, Ji Chan, Park, Hyung Ju
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9960270/
https://www.ncbi.nlm.nih.gov/pubmed/36839027
http://dx.doi.org/10.3390/nano13040659
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author Jeon, Seung Jin
Oh, Kyung Hee
Choi, Youngbo
Park, Ji Chan
Park, Hyung Ju
author_facet Jeon, Seung Jin
Oh, Kyung Hee
Choi, Youngbo
Park, Ji Chan
Park, Hyung Ju
author_sort Jeon, Seung Jin
collection PubMed
description Highly dispersed Pt-incorporated mesoporous Fe(2)O(3) (Pt/m-Fe(2)O(3)) of 4 μm size is prepared through a simple hydrothermal reaction and thermal decomposition procedures. Furthermore, the formaldehyde gas-sensing properties of Pt/m-Fe(2)O(3) are investigated. Compared with our previous mesoporous Fe(2)O(3)-based gas sensors, a gas sensor based on 0.2% Pt/m-Fe(2)O(3) shows improved gas response by over 90% in detecting low-level formaldehyde gas at 50 ppb concentration, an enhanced selectivity of formaldehyde gas, and a lower degradation of sensing performance in high-humidity environments. Additionally, the gas sensor exhibits similar properties as the previous sensor, such as operating temperature (275 °C) and long-term stability. The enhancement in formaldehyde gas-sensing performance is attributed to the attractive catalytic chemical sensitization of highly dispersed Pt nanoparticles in the mesoporous Fe(2)O(3) microcube architecture.
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spelling pubmed-99602702023-02-26 Highly Dispersed Pt-Incorporated Mesoporous Fe(2)O(3) for Low-Level Sensing of Formaldehyde Gas Jeon, Seung Jin Oh, Kyung Hee Choi, Youngbo Park, Ji Chan Park, Hyung Ju Nanomaterials (Basel) Article Highly dispersed Pt-incorporated mesoporous Fe(2)O(3) (Pt/m-Fe(2)O(3)) of 4 μm size is prepared through a simple hydrothermal reaction and thermal decomposition procedures. Furthermore, the formaldehyde gas-sensing properties of Pt/m-Fe(2)O(3) are investigated. Compared with our previous mesoporous Fe(2)O(3)-based gas sensors, a gas sensor based on 0.2% Pt/m-Fe(2)O(3) shows improved gas response by over 90% in detecting low-level formaldehyde gas at 50 ppb concentration, an enhanced selectivity of formaldehyde gas, and a lower degradation of sensing performance in high-humidity environments. Additionally, the gas sensor exhibits similar properties as the previous sensor, such as operating temperature (275 °C) and long-term stability. The enhancement in formaldehyde gas-sensing performance is attributed to the attractive catalytic chemical sensitization of highly dispersed Pt nanoparticles in the mesoporous Fe(2)O(3) microcube architecture. MDPI 2023-02-08 /pmc/articles/PMC9960270/ /pubmed/36839027 http://dx.doi.org/10.3390/nano13040659 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Jeon, Seung Jin
Oh, Kyung Hee
Choi, Youngbo
Park, Ji Chan
Park, Hyung Ju
Highly Dispersed Pt-Incorporated Mesoporous Fe(2)O(3) for Low-Level Sensing of Formaldehyde Gas
title Highly Dispersed Pt-Incorporated Mesoporous Fe(2)O(3) for Low-Level Sensing of Formaldehyde Gas
title_full Highly Dispersed Pt-Incorporated Mesoporous Fe(2)O(3) for Low-Level Sensing of Formaldehyde Gas
title_fullStr Highly Dispersed Pt-Incorporated Mesoporous Fe(2)O(3) for Low-Level Sensing of Formaldehyde Gas
title_full_unstemmed Highly Dispersed Pt-Incorporated Mesoporous Fe(2)O(3) for Low-Level Sensing of Formaldehyde Gas
title_short Highly Dispersed Pt-Incorporated Mesoporous Fe(2)O(3) for Low-Level Sensing of Formaldehyde Gas
title_sort highly dispersed pt-incorporated mesoporous fe(2)o(3) for low-level sensing of formaldehyde gas
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9960270/
https://www.ncbi.nlm.nih.gov/pubmed/36839027
http://dx.doi.org/10.3390/nano13040659
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