Damping under Varying Frequencies, Mechanical Properties, and Failure Modes of Flax/Polypropylene Composites

This work investigates the effects of fibre content, fibre orientation, and frequency on the dynamic behaviour of flax fibre-reinforced polypropylene composites (FFPCs) to improve understanding of the parameters affecting vibration damping in FFPCs. The effects of fibre content and fibre orientation on the mechanical performances of FFPCs, along with fracture characteristics, are also investigated in this study. Laminates of various fibre contents and orientations were manufactured by a vacuum bagging process, and their dynamic and static properties were then obtained using dynamic (dynamic mechanical analysis (DMA) to frequencies of 100 Hz) and various mechanical (tensile and flexural) analyses, respectively. The findings suggest that of all the parameters, fibre orientation has the most significant impact on the damping, and the maximum loss factor (i.e., 4.3–5.5%) is obtained for 45° and 60° fibre orientations. However, there is no significant difference in loss factors among the composites with different fibre contents. The loss factors lie mainly in the range of 4–5.5%, irrespective of the fibre volume fraction, fibre orientation, and frequency. A significant improvement (281 to 953%) in damping is feasible in flax fibre/polypropylene composites relative to more widespread glass/epoxy composites. The mechanical properties of composites are also strongly affected by fibre orientation with respect to the loading direction; for example, the tensile modulus decreases from 20 GPa to 3.45 GPa at an off-axis angle of 30° for a fibre volume fraction of 0.40. The largest mechanical properties (tensile and flexural) are found in the case of 0° fibre orientation. For composites with fibre volume fractions in the range 0.31–0.50, tensile moduli are in the range 16–21 GPa, and tensile strengths are in the range 125–173 MPa, while flexural moduli and strengths are in the ranges 12–15 GPa and 96–121 MPa, respectively, making them suitable for structural applications. The obtained results also suggest that flax fibre composites are comparable to glass fibre composites, especially in terms of specific stiffness. The ESEM analysis confirms the tensile failures of specimens due to fibre debonding, fibre pull-out and breakage, matrix cracking, and inadequate fibre/matrix adhesion. The outcomes from this study indicate that flax fibre-reinforced composite could be a commercially viable material for applications in which noise and vibration are significant issues and where a significant amount of damping is required with a combination of high stiffness and low weight.