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Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields

Using an ab initio, time-dependent calculational method, we study the non-linear dynamics of a two-electron quantum dot in the presence of ultrashort Thz laser pulses. The analysis of the contribution of the various partial waves to two-electron joint radial and energy distribution patterns revealed...

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Detalles Bibliográficos
Autores principales: Prior, Adam, Nikolopoulos, Lampros A. A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9967998/
https://www.ncbi.nlm.nih.gov/pubmed/36837035
http://dx.doi.org/10.3390/ma16041405
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author Prior, Adam
Nikolopoulos, Lampros A. A.
author_facet Prior, Adam
Nikolopoulos, Lampros A. A.
author_sort Prior, Adam
collection PubMed
description Using an ab initio, time-dependent calculational method, we study the non-linear dynamics of a two-electron quantum dot in the presence of ultrashort Thz laser pulses. The analysis of the contribution of the various partial waves to two-electron joint radial and energy distribution patterns revealed strongly correlated electron ejection channels. In the double-ionization process, regardless of the photon energy, the two-electron wave packets are born and remain concentrated until the pulse’s peak; at later times, and depending on the photon energy of the field, distinctly different patterns emerge. Our calculations also showed the gradual transition of the radial and energy patterns from a single-peak to a doubly peaked structure, associated with the direct and the sequential double-ionization mechanisms, respectively.
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spelling pubmed-99679982023-02-27 Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields Prior, Adam Nikolopoulos, Lampros A. A. Materials (Basel) Article Using an ab initio, time-dependent calculational method, we study the non-linear dynamics of a two-electron quantum dot in the presence of ultrashort Thz laser pulses. The analysis of the contribution of the various partial waves to two-electron joint radial and energy distribution patterns revealed strongly correlated electron ejection channels. In the double-ionization process, regardless of the photon energy, the two-electron wave packets are born and remain concentrated until the pulse’s peak; at later times, and depending on the photon energy of the field, distinctly different patterns emerge. Our calculations also showed the gradual transition of the radial and energy patterns from a single-peak to a doubly peaked structure, associated with the direct and the sequential double-ionization mechanisms, respectively. MDPI 2023-02-07 /pmc/articles/PMC9967998/ /pubmed/36837035 http://dx.doi.org/10.3390/ma16041405 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Prior, Adam
Nikolopoulos, Lampros A. A.
Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields
title Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields
title_full Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields
title_fullStr Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields
title_full_unstemmed Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields
title_short Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields
title_sort dynamics of correlated double-ionization of two-electron quantum dots in laser fields
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9967998/
https://www.ncbi.nlm.nih.gov/pubmed/36837035
http://dx.doi.org/10.3390/ma16041405
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