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Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields
Using an ab initio, time-dependent calculational method, we study the non-linear dynamics of a two-electron quantum dot in the presence of ultrashort Thz laser pulses. The analysis of the contribution of the various partial waves to two-electron joint radial and energy distribution patterns revealed...
Autores principales: | , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9967998/ https://www.ncbi.nlm.nih.gov/pubmed/36837035 http://dx.doi.org/10.3390/ma16041405 |
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author | Prior, Adam Nikolopoulos, Lampros A. A. |
author_facet | Prior, Adam Nikolopoulos, Lampros A. A. |
author_sort | Prior, Adam |
collection | PubMed |
description | Using an ab initio, time-dependent calculational method, we study the non-linear dynamics of a two-electron quantum dot in the presence of ultrashort Thz laser pulses. The analysis of the contribution of the various partial waves to two-electron joint radial and energy distribution patterns revealed strongly correlated electron ejection channels. In the double-ionization process, regardless of the photon energy, the two-electron wave packets are born and remain concentrated until the pulse’s peak; at later times, and depending on the photon energy of the field, distinctly different patterns emerge. Our calculations also showed the gradual transition of the radial and energy patterns from a single-peak to a doubly peaked structure, associated with the direct and the sequential double-ionization mechanisms, respectively. |
format | Online Article Text |
id | pubmed-9967998 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-99679982023-02-27 Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields Prior, Adam Nikolopoulos, Lampros A. A. Materials (Basel) Article Using an ab initio, time-dependent calculational method, we study the non-linear dynamics of a two-electron quantum dot in the presence of ultrashort Thz laser pulses. The analysis of the contribution of the various partial waves to two-electron joint radial and energy distribution patterns revealed strongly correlated electron ejection channels. In the double-ionization process, regardless of the photon energy, the two-electron wave packets are born and remain concentrated until the pulse’s peak; at later times, and depending on the photon energy of the field, distinctly different patterns emerge. Our calculations also showed the gradual transition of the radial and energy patterns from a single-peak to a doubly peaked structure, associated with the direct and the sequential double-ionization mechanisms, respectively. MDPI 2023-02-07 /pmc/articles/PMC9967998/ /pubmed/36837035 http://dx.doi.org/10.3390/ma16041405 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Prior, Adam Nikolopoulos, Lampros A. A. Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields |
title | Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields |
title_full | Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields |
title_fullStr | Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields |
title_full_unstemmed | Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields |
title_short | Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields |
title_sort | dynamics of correlated double-ionization of two-electron quantum dots in laser fields |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9967998/ https://www.ncbi.nlm.nih.gov/pubmed/36837035 http://dx.doi.org/10.3390/ma16041405 |
work_keys_str_mv | AT prioradam dynamicsofcorrelateddoubleionizationoftwoelectronquantumdotsinlaserfields AT nikolopouloslamprosaa dynamicsofcorrelateddoubleionizationoftwoelectronquantumdotsinlaserfields |