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Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline
In this paper, with the help of the method of composite materials science, parallel synthesis and high-throughput screening were used to prepare gas sensors with different molar ratios of rare earths and precious metals modified In(2)O(3), which could be used to monitor and warn the early leakage of...
Autores principales: | , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9968188/ https://www.ncbi.nlm.nih.gov/pubmed/36837145 http://dx.doi.org/10.3390/ma16041517 |
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author | Zhang, Deqi Guo, Shenghui Gao, Jiyun Yang, Li Zhu, Ye Ma, Yanjia Hou, Ming |
author_facet | Zhang, Deqi Guo, Shenghui Gao, Jiyun Yang, Li Zhu, Ye Ma, Yanjia Hou, Ming |
author_sort | Zhang, Deqi |
collection | PubMed |
description | In this paper, with the help of the method of composite materials science, parallel synthesis and high-throughput screening were used to prepare gas sensors with different molar ratios of rare earths and precious metals modified In(2)O(3), which could be used to monitor and warn the early leakage of gasoline and diesel. Through high-throughput screening, it is found that the effect of rare earth metal modification on gas sensitivity improvement is better than other metals, especially 0.5 mol% Gd modified In(2)O(3) (Gd(0.5)In) gas sensor has a high response to 100 ppm gasoline (R(a)/R(g) = 6.1) and diesel (R(a)/R(g) = 5) volatiles at 250 °C. Compared with the existing literature, the sensor has low detection concentration and suitable stability. This is mainly due to the alteration of surface chemisorption oxygen caused by the catalysis and modification of rare earth itself. |
format | Online Article Text |
id | pubmed-9968188 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-99681882023-02-27 Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline Zhang, Deqi Guo, Shenghui Gao, Jiyun Yang, Li Zhu, Ye Ma, Yanjia Hou, Ming Materials (Basel) Article In this paper, with the help of the method of composite materials science, parallel synthesis and high-throughput screening were used to prepare gas sensors with different molar ratios of rare earths and precious metals modified In(2)O(3), which could be used to monitor and warn the early leakage of gasoline and diesel. Through high-throughput screening, it is found that the effect of rare earth metal modification on gas sensitivity improvement is better than other metals, especially 0.5 mol% Gd modified In(2)O(3) (Gd(0.5)In) gas sensor has a high response to 100 ppm gasoline (R(a)/R(g) = 6.1) and diesel (R(a)/R(g) = 5) volatiles at 250 °C. Compared with the existing literature, the sensor has low detection concentration and suitable stability. This is mainly due to the alteration of surface chemisorption oxygen caused by the catalysis and modification of rare earth itself. MDPI 2023-02-11 /pmc/articles/PMC9968188/ /pubmed/36837145 http://dx.doi.org/10.3390/ma16041517 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Zhang, Deqi Guo, Shenghui Gao, Jiyun Yang, Li Zhu, Ye Ma, Yanjia Hou, Ming Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline |
title | Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline |
title_full | Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline |
title_fullStr | Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline |
title_full_unstemmed | Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline |
title_short | Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline |
title_sort | surface-modified in(2)o(3) for high-throughput screening of volatile gas sensors in diesel and gasoline |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9968188/ https://www.ncbi.nlm.nih.gov/pubmed/36837145 http://dx.doi.org/10.3390/ma16041517 |
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