Cargando…

Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline

In this paper, with the help of the method of composite materials science, parallel synthesis and high-throughput screening were used to prepare gas sensors with different molar ratios of rare earths and precious metals modified In(2)O(3), which could be used to monitor and warn the early leakage of...

Descripción completa

Detalles Bibliográficos
Autores principales: Zhang, Deqi, Guo, Shenghui, Gao, Jiyun, Yang, Li, Zhu, Ye, Ma, Yanjia, Hou, Ming
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9968188/
https://www.ncbi.nlm.nih.gov/pubmed/36837145
http://dx.doi.org/10.3390/ma16041517
_version_ 1784897452414861312
author Zhang, Deqi
Guo, Shenghui
Gao, Jiyun
Yang, Li
Zhu, Ye
Ma, Yanjia
Hou, Ming
author_facet Zhang, Deqi
Guo, Shenghui
Gao, Jiyun
Yang, Li
Zhu, Ye
Ma, Yanjia
Hou, Ming
author_sort Zhang, Deqi
collection PubMed
description In this paper, with the help of the method of composite materials science, parallel synthesis and high-throughput screening were used to prepare gas sensors with different molar ratios of rare earths and precious metals modified In(2)O(3), which could be used to monitor and warn the early leakage of gasoline and diesel. Through high-throughput screening, it is found that the effect of rare earth metal modification on gas sensitivity improvement is better than other metals, especially 0.5 mol% Gd modified In(2)O(3) (Gd(0.5)In) gas sensor has a high response to 100 ppm gasoline (R(a)/R(g) = 6.1) and diesel (R(a)/R(g) = 5) volatiles at 250 °C. Compared with the existing literature, the sensor has low detection concentration and suitable stability. This is mainly due to the alteration of surface chemisorption oxygen caused by the catalysis and modification of rare earth itself.
format Online
Article
Text
id pubmed-9968188
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher MDPI
record_format MEDLINE/PubMed
spelling pubmed-99681882023-02-27 Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline Zhang, Deqi Guo, Shenghui Gao, Jiyun Yang, Li Zhu, Ye Ma, Yanjia Hou, Ming Materials (Basel) Article In this paper, with the help of the method of composite materials science, parallel synthesis and high-throughput screening were used to prepare gas sensors with different molar ratios of rare earths and precious metals modified In(2)O(3), which could be used to monitor and warn the early leakage of gasoline and diesel. Through high-throughput screening, it is found that the effect of rare earth metal modification on gas sensitivity improvement is better than other metals, especially 0.5 mol% Gd modified In(2)O(3) (Gd(0.5)In) gas sensor has a high response to 100 ppm gasoline (R(a)/R(g) = 6.1) and diesel (R(a)/R(g) = 5) volatiles at 250 °C. Compared with the existing literature, the sensor has low detection concentration and suitable stability. This is mainly due to the alteration of surface chemisorption oxygen caused by the catalysis and modification of rare earth itself. MDPI 2023-02-11 /pmc/articles/PMC9968188/ /pubmed/36837145 http://dx.doi.org/10.3390/ma16041517 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Zhang, Deqi
Guo, Shenghui
Gao, Jiyun
Yang, Li
Zhu, Ye
Ma, Yanjia
Hou, Ming
Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline
title Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline
title_full Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline
title_fullStr Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline
title_full_unstemmed Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline
title_short Surface-Modified In(2)O(3) for High-Throughput Screening of Volatile Gas Sensors in Diesel and Gasoline
title_sort surface-modified in(2)o(3) for high-throughput screening of volatile gas sensors in diesel and gasoline
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9968188/
https://www.ncbi.nlm.nih.gov/pubmed/36837145
http://dx.doi.org/10.3390/ma16041517
work_keys_str_mv AT zhangdeqi surfacemodifiedin2o3forhighthroughputscreeningofvolatilegassensorsindieselandgasoline
AT guoshenghui surfacemodifiedin2o3forhighthroughputscreeningofvolatilegassensorsindieselandgasoline
AT gaojiyun surfacemodifiedin2o3forhighthroughputscreeningofvolatilegassensorsindieselandgasoline
AT yangli surfacemodifiedin2o3forhighthroughputscreeningofvolatilegassensorsindieselandgasoline
AT zhuye surfacemodifiedin2o3forhighthroughputscreeningofvolatilegassensorsindieselandgasoline
AT mayanjia surfacemodifiedin2o3forhighthroughputscreeningofvolatilegassensorsindieselandgasoline
AT houming surfacemodifiedin2o3forhighthroughputscreeningofvolatilegassensorsindieselandgasoline