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Viscoelastic coarsening of quasi-2D foam

Foams are unstable jammed materials. They evolve over timescales comparable to their “time of use", which makes the study of their destabilisation mechanisms crucial for applications. In practice, many foams are made from viscoelastic fluids, which are observed to prolong their lifetimes. Despi...

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Autores principales: Guidolin, Chiara, Mac Intyre, Jonatan, Rio, Emmanuelle, Puisto, Antti, Salonen, Anniina
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9975196/
https://www.ncbi.nlm.nih.gov/pubmed/36854671
http://dx.doi.org/10.1038/s41467-023-36763-y
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author Guidolin, Chiara
Mac Intyre, Jonatan
Rio, Emmanuelle
Puisto, Antti
Salonen, Anniina
author_facet Guidolin, Chiara
Mac Intyre, Jonatan
Rio, Emmanuelle
Puisto, Antti
Salonen, Anniina
author_sort Guidolin, Chiara
collection PubMed
description Foams are unstable jammed materials. They evolve over timescales comparable to their “time of use", which makes the study of their destabilisation mechanisms crucial for applications. In practice, many foams are made from viscoelastic fluids, which are observed to prolong their lifetimes. Despite their importance, we lack understanding of the coarsening mechanism in such systems. We probe the effect of continuous phase viscoelasticity on foam coarsening with foamed emulsions. We show that bubble size evolution is strongly slowed down and foam structure hugely impacted. The main mechanisms responsible are the absence of continuous phase redistribution and a non-trivial link between foam structure and mechanical properties. These combine to give spatially heterogeneous coarsening. Beyond their importance in the design of foamy materials, the results give a macroscopic vision of phase separation in a viscoelastic medium.
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spelling pubmed-99751962023-03-02 Viscoelastic coarsening of quasi-2D foam Guidolin, Chiara Mac Intyre, Jonatan Rio, Emmanuelle Puisto, Antti Salonen, Anniina Nat Commun Article Foams are unstable jammed materials. They evolve over timescales comparable to their “time of use", which makes the study of their destabilisation mechanisms crucial for applications. In practice, many foams are made from viscoelastic fluids, which are observed to prolong their lifetimes. Despite their importance, we lack understanding of the coarsening mechanism in such systems. We probe the effect of continuous phase viscoelasticity on foam coarsening with foamed emulsions. We show that bubble size evolution is strongly slowed down and foam structure hugely impacted. The main mechanisms responsible are the absence of continuous phase redistribution and a non-trivial link between foam structure and mechanical properties. These combine to give spatially heterogeneous coarsening. Beyond their importance in the design of foamy materials, the results give a macroscopic vision of phase separation in a viscoelastic medium. Nature Publishing Group UK 2023-02-28 /pmc/articles/PMC9975196/ /pubmed/36854671 http://dx.doi.org/10.1038/s41467-023-36763-y Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Guidolin, Chiara
Mac Intyre, Jonatan
Rio, Emmanuelle
Puisto, Antti
Salonen, Anniina
Viscoelastic coarsening of quasi-2D foam
title Viscoelastic coarsening of quasi-2D foam
title_full Viscoelastic coarsening of quasi-2D foam
title_fullStr Viscoelastic coarsening of quasi-2D foam
title_full_unstemmed Viscoelastic coarsening of quasi-2D foam
title_short Viscoelastic coarsening of quasi-2D foam
title_sort viscoelastic coarsening of quasi-2d foam
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9975196/
https://www.ncbi.nlm.nih.gov/pubmed/36854671
http://dx.doi.org/10.1038/s41467-023-36763-y
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