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Simulation Study on the Interaction between Chemically Reacting Double Coal Char Particles

[Image: see text] Due to the complex atmosphere of the entrained flow gasifier, it is difficult to obtain reactivity properties of coal char particles under high-temperature conditions by experiment. The computational fluid dynamics simulation method is a key way to simulate the reactivity of coal c...

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Autores principales: Su, Weiguang, Shi, Meiyu, Zhang, Ben, Wang, Wenxin, Song, Xudong, Yu, Guangsuo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9979330/
https://www.ncbi.nlm.nih.gov/pubmed/36872985
http://dx.doi.org/10.1021/acsomega.2c07675
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author Su, Weiguang
Shi, Meiyu
Zhang, Ben
Wang, Wenxin
Song, Xudong
Yu, Guangsuo
author_facet Su, Weiguang
Shi, Meiyu
Zhang, Ben
Wang, Wenxin
Song, Xudong
Yu, Guangsuo
author_sort Su, Weiguang
collection PubMed
description [Image: see text] Due to the complex atmosphere of the entrained flow gasifier, it is difficult to obtain reactivity properties of coal char particles under high-temperature conditions by experiment. The computational fluid dynamics simulation method is a key way to simulate the reactivity of coal char particles. In this article, the gasification characteristics of double coal char particles under H(2)O/O(2)/CO(2) atmosphere are studied. The results show that the particle distance (L) has an influence on the reaction with particles. With the gradual increase of L, the temperature first rises and then falls among the double particles due to the migration of the reaction area, and the characteristics of double coal char particles gradually approach that of single coal char particles. The particle size also has an influence on the gasification characteristics of coal char particles. As the particle size varies from 0.1 to 1 mm, the reaction area of particles becomes smaller at high temperature and finally attaches to the surface of the particles. The reaction rate and carbon consumption rate increase with increasing particle size. As the size of double particles is changed, the reaction rate trend of double coal char particles at the same particle distance is basically the same, but the change degree of reaction rate is different. With the increase of the distance between coal char particles, the change of the carbon consumption rate is larger for the small particle size.
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spelling pubmed-99793302023-03-03 Simulation Study on the Interaction between Chemically Reacting Double Coal Char Particles Su, Weiguang Shi, Meiyu Zhang, Ben Wang, Wenxin Song, Xudong Yu, Guangsuo ACS Omega [Image: see text] Due to the complex atmosphere of the entrained flow gasifier, it is difficult to obtain reactivity properties of coal char particles under high-temperature conditions by experiment. The computational fluid dynamics simulation method is a key way to simulate the reactivity of coal char particles. In this article, the gasification characteristics of double coal char particles under H(2)O/O(2)/CO(2) atmosphere are studied. The results show that the particle distance (L) has an influence on the reaction with particles. With the gradual increase of L, the temperature first rises and then falls among the double particles due to the migration of the reaction area, and the characteristics of double coal char particles gradually approach that of single coal char particles. The particle size also has an influence on the gasification characteristics of coal char particles. As the particle size varies from 0.1 to 1 mm, the reaction area of particles becomes smaller at high temperature and finally attaches to the surface of the particles. The reaction rate and carbon consumption rate increase with increasing particle size. As the size of double particles is changed, the reaction rate trend of double coal char particles at the same particle distance is basically the same, but the change degree of reaction rate is different. With the increase of the distance between coal char particles, the change of the carbon consumption rate is larger for the small particle size. American Chemical Society 2023-02-14 /pmc/articles/PMC9979330/ /pubmed/36872985 http://dx.doi.org/10.1021/acsomega.2c07675 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Su, Weiguang
Shi, Meiyu
Zhang, Ben
Wang, Wenxin
Song, Xudong
Yu, Guangsuo
Simulation Study on the Interaction between Chemically Reacting Double Coal Char Particles
title Simulation Study on the Interaction between Chemically Reacting Double Coal Char Particles
title_full Simulation Study on the Interaction between Chemically Reacting Double Coal Char Particles
title_fullStr Simulation Study on the Interaction between Chemically Reacting Double Coal Char Particles
title_full_unstemmed Simulation Study on the Interaction between Chemically Reacting Double Coal Char Particles
title_short Simulation Study on the Interaction between Chemically Reacting Double Coal Char Particles
title_sort simulation study on the interaction between chemically reacting double coal char particles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9979330/
https://www.ncbi.nlm.nih.gov/pubmed/36872985
http://dx.doi.org/10.1021/acsomega.2c07675
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