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Effect of ions on sulfuric acid-water binary particle formation: 1. Theory for kinetic- and nucleation-type particle formation and atmospheric implications

We derive a version of Classical Nucleation Theory normalized by quantum chemical results on sulfuric acid-water hydration to describe neutral and ion-induced particle formation in the binary sulfuric acid-water system. The theory is extended to treat the kinetic regime where the nucleation free ene...

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Detalles Bibliográficos
Autores principales: Merikanto, Joonas, Duplissy, Jonathan, Määttänen, Anni, Henschel, Henning, Donahue, Neil M, Brus, David, Schobesberger, Siegfried, Kulmala, Markku, Vehkamäki, Hanna
Lenguaje:eng
Publicado: 2016
Materias:
Acceso en línea:https://dx.doi.org/10.1002/2015JD023538
http://cds.cern.ch/record/2291602