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Effect of ions on sulfuric acid-water binary particle formation: 1. Theory for kinetic- and nucleation-type particle formation and atmospheric implications
We derive a version of Classical Nucleation Theory normalized by quantum chemical results on sulfuric acid-water hydration to describe neutral and ion-induced particle formation in the binary sulfuric acid-water system. The theory is extended to treat the kinetic regime where the nucleation free ene...
Autores principales: | Merikanto, Joonas, Duplissy, Jonathan, Määttänen, Anni, Henschel, Henning, Donahue, Neil M, Brus, David, Schobesberger, Siegfried, Kulmala, Markku, Vehkamäki, Hanna |
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Lenguaje: | eng |
Publicado: |
2016
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Materias: | |
Acceso en línea: | https://dx.doi.org/10.1002/2015JD023538 http://cds.cern.ch/record/2291602 |
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