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Enhancement of the Electroluminescence from Amorphous Er-Doped Al(2)O(3) Nanolaminate Films by Y(2)O(3) Cladding Layers Using Atomic Layer Deposition

Amorphous Al(2)O(3)-Y(2)O(3):Er nanolaminate films are fabricated on silicon by atomic layer deposition, and ~1530 nm electroluminescence (EL) is obtained from the metal-oxide-semiconductor light-emitting devices based on these nanofilms. The introduction of Y(2)O(3) into Al(2)O(3) reduces the elect...

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Detalles Bibliográficos
Autores principales: Yang, Yang, Pei, Haiyan, Ye, Zejun, Sun, Jiaming
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10005131/
https://www.ncbi.nlm.nih.gov/pubmed/36903727
http://dx.doi.org/10.3390/nano13050849
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author Yang, Yang
Pei, Haiyan
Ye, Zejun
Sun, Jiaming
author_facet Yang, Yang
Pei, Haiyan
Ye, Zejun
Sun, Jiaming
author_sort Yang, Yang
collection PubMed
description Amorphous Al(2)O(3)-Y(2)O(3):Er nanolaminate films are fabricated on silicon by atomic layer deposition, and ~1530 nm electroluminescence (EL) is obtained from the metal-oxide-semiconductor light-emitting devices based on these nanofilms. The introduction of Y(2)O(3) into Al(2)O(3) reduces the electric field for Er excitation and the EL performance is significantly enhanced, while the electron injection of devices and the radiative recombination of doped Er(3+) ions are not impacted. The 0.2 nm Y(2)O(3) cladding layers for Er(3+) ions increase the external quantum efficiency from ~3% to 8.7% and the power efficiency is increased by nearly one order of magnitude to 0.12%. The EL is ascribed to the impact excitation of Er(3+) ions by hot electrons, which stem from Poole-Frenkel conduction mechanism under sufficient voltage within the Al(2)O(3)-Y(2)O(3) matrix.
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spelling pubmed-100051312023-03-11 Enhancement of the Electroluminescence from Amorphous Er-Doped Al(2)O(3) Nanolaminate Films by Y(2)O(3) Cladding Layers Using Atomic Layer Deposition Yang, Yang Pei, Haiyan Ye, Zejun Sun, Jiaming Nanomaterials (Basel) Article Amorphous Al(2)O(3)-Y(2)O(3):Er nanolaminate films are fabricated on silicon by atomic layer deposition, and ~1530 nm electroluminescence (EL) is obtained from the metal-oxide-semiconductor light-emitting devices based on these nanofilms. The introduction of Y(2)O(3) into Al(2)O(3) reduces the electric field for Er excitation and the EL performance is significantly enhanced, while the electron injection of devices and the radiative recombination of doped Er(3+) ions are not impacted. The 0.2 nm Y(2)O(3) cladding layers for Er(3+) ions increase the external quantum efficiency from ~3% to 8.7% and the power efficiency is increased by nearly one order of magnitude to 0.12%. The EL is ascribed to the impact excitation of Er(3+) ions by hot electrons, which stem from Poole-Frenkel conduction mechanism under sufficient voltage within the Al(2)O(3)-Y(2)O(3) matrix. MDPI 2023-02-24 /pmc/articles/PMC10005131/ /pubmed/36903727 http://dx.doi.org/10.3390/nano13050849 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Yang, Yang
Pei, Haiyan
Ye, Zejun
Sun, Jiaming
Enhancement of the Electroluminescence from Amorphous Er-Doped Al(2)O(3) Nanolaminate Films by Y(2)O(3) Cladding Layers Using Atomic Layer Deposition
title Enhancement of the Electroluminescence from Amorphous Er-Doped Al(2)O(3) Nanolaminate Films by Y(2)O(3) Cladding Layers Using Atomic Layer Deposition
title_full Enhancement of the Electroluminescence from Amorphous Er-Doped Al(2)O(3) Nanolaminate Films by Y(2)O(3) Cladding Layers Using Atomic Layer Deposition
title_fullStr Enhancement of the Electroluminescence from Amorphous Er-Doped Al(2)O(3) Nanolaminate Films by Y(2)O(3) Cladding Layers Using Atomic Layer Deposition
title_full_unstemmed Enhancement of the Electroluminescence from Amorphous Er-Doped Al(2)O(3) Nanolaminate Films by Y(2)O(3) Cladding Layers Using Atomic Layer Deposition
title_short Enhancement of the Electroluminescence from Amorphous Er-Doped Al(2)O(3) Nanolaminate Films by Y(2)O(3) Cladding Layers Using Atomic Layer Deposition
title_sort enhancement of the electroluminescence from amorphous er-doped al(2)o(3) nanolaminate films by y(2)o(3) cladding layers using atomic layer deposition
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10005131/
https://www.ncbi.nlm.nih.gov/pubmed/36903727
http://dx.doi.org/10.3390/nano13050849
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