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Direct observation of coherence transfer and rotational-to-vibrational energy exchange in optically centrifuged CO(2) super-rotors

Optical centrifuges are laser-based molecular traps that can rotationally accelerate molecules to energies rivalling or exceeding molecular bond energies. Here we report time and frequency-resolved ultrafast coherent Raman measurements of optically centrifuged CO(2) at 380 Torr spun to energies beyo...

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Detalles Bibliográficos
Autores principales: Chen, Timothy Y., Steinmetz, Scott A., Patterson, Brian D., Jasper, Ahren W., Kliewer, Christopher J.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10239519/
https://www.ncbi.nlm.nih.gov/pubmed/37270647
http://dx.doi.org/10.1038/s41467-023-38873-z