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UO(2) dissolution in bicarbonate solution with H(2)O(2): the effect of temperature

Upon nuclear waste canister failure and contact of spent nuclear fuel with groundwater, the UO(2) matrix of spent fuel will interact with oxidants in the groundwater generated by water radiolysis. Bicarbonate (HCO(3)(−)) is often found in groundwater, and the H(2)O(2) induced oxidative dissolution o...

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Detalles Bibliográficos
Autores principales: McGrady, John, Kumagai, Yuta, Kitatsuji, Yoshihiro, Kirishima, Akira, Akiyama, Daisuke, Watanabe, Masayuki
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10517105/
https://www.ncbi.nlm.nih.gov/pubmed/37746334
http://dx.doi.org/10.1039/d2ra08131h