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Investigation of the Impact of Point Defects in InGaN/GaN Quantum Wells with High Dislocation Densities

In this work, we report on the efficiency of single InGaN/GaN quantum wells (QWs) grown on thin (<1 µm) GaN buffer layers on silicon (111) substrates exhibiting very high threading dislocation (TD) densities. Despite this high defect density, we show that QW emission efficiency significantly incr...

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Autores principales: Lottigier, Pierre, Di Paola, Davide Maria, Alexander, Duncan T. L., Weatherley, Thomas F. K., Sáenz de Santa María Modroño, Pablo, Chen, Danxuan, Jacopin, Gwénolé, Carlin, Jean-François, Butté, Raphaël, Grandjean, Nicolas
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10537355/
https://www.ncbi.nlm.nih.gov/pubmed/37764598
http://dx.doi.org/10.3390/nano13182569
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author Lottigier, Pierre
Di Paola, Davide Maria
Alexander, Duncan T. L.
Weatherley, Thomas F. K.
Sáenz de Santa María Modroño, Pablo
Chen, Danxuan
Jacopin, Gwénolé
Carlin, Jean-François
Butté, Raphaël
Grandjean, Nicolas
author_facet Lottigier, Pierre
Di Paola, Davide Maria
Alexander, Duncan T. L.
Weatherley, Thomas F. K.
Sáenz de Santa María Modroño, Pablo
Chen, Danxuan
Jacopin, Gwénolé
Carlin, Jean-François
Butté, Raphaël
Grandjean, Nicolas
author_sort Lottigier, Pierre
collection PubMed
description In this work, we report on the efficiency of single InGaN/GaN quantum wells (QWs) grown on thin (<1 µm) GaN buffer layers on silicon (111) substrates exhibiting very high threading dislocation (TD) densities. Despite this high defect density, we show that QW emission efficiency significantly increases upon the insertion of an In-containing underlayer, whose role is to prevent the introduction of point defects during the growth of InGaN QWs. Hence, we demonstrate that point defects play a key role in limiting InGaN QW efficiency, even in samples where their density (2–3 × 10 [Formula: see text] cm [Formula: see text]) is much lower than that of TD (2–3 × 10 [Formula: see text] cm [Formula: see text]). Time-resolved photoluminescence and cathodoluminescence studies confirm the prevalence of point defects over TDs in QW efficiency. Interestingly, TD terminations lead to the formation of independent domains for carriers, thanks to V-pits and step bunching phenomena.
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spelling pubmed-105373552023-09-29 Investigation of the Impact of Point Defects in InGaN/GaN Quantum Wells with High Dislocation Densities Lottigier, Pierre Di Paola, Davide Maria Alexander, Duncan T. L. Weatherley, Thomas F. K. Sáenz de Santa María Modroño, Pablo Chen, Danxuan Jacopin, Gwénolé Carlin, Jean-François Butté, Raphaël Grandjean, Nicolas Nanomaterials (Basel) Article In this work, we report on the efficiency of single InGaN/GaN quantum wells (QWs) grown on thin (<1 µm) GaN buffer layers on silicon (111) substrates exhibiting very high threading dislocation (TD) densities. Despite this high defect density, we show that QW emission efficiency significantly increases upon the insertion of an In-containing underlayer, whose role is to prevent the introduction of point defects during the growth of InGaN QWs. Hence, we demonstrate that point defects play a key role in limiting InGaN QW efficiency, even in samples where their density (2–3 × 10 [Formula: see text] cm [Formula: see text]) is much lower than that of TD (2–3 × 10 [Formula: see text] cm [Formula: see text]). Time-resolved photoluminescence and cathodoluminescence studies confirm the prevalence of point defects over TDs in QW efficiency. Interestingly, TD terminations lead to the formation of independent domains for carriers, thanks to V-pits and step bunching phenomena. MDPI 2023-09-16 /pmc/articles/PMC10537355/ /pubmed/37764598 http://dx.doi.org/10.3390/nano13182569 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Lottigier, Pierre
Di Paola, Davide Maria
Alexander, Duncan T. L.
Weatherley, Thomas F. K.
Sáenz de Santa María Modroño, Pablo
Chen, Danxuan
Jacopin, Gwénolé
Carlin, Jean-François
Butté, Raphaël
Grandjean, Nicolas
Investigation of the Impact of Point Defects in InGaN/GaN Quantum Wells with High Dislocation Densities
title Investigation of the Impact of Point Defects in InGaN/GaN Quantum Wells with High Dislocation Densities
title_full Investigation of the Impact of Point Defects in InGaN/GaN Quantum Wells with High Dislocation Densities
title_fullStr Investigation of the Impact of Point Defects in InGaN/GaN Quantum Wells with High Dislocation Densities
title_full_unstemmed Investigation of the Impact of Point Defects in InGaN/GaN Quantum Wells with High Dislocation Densities
title_short Investigation of the Impact of Point Defects in InGaN/GaN Quantum Wells with High Dislocation Densities
title_sort investigation of the impact of point defects in ingan/gan quantum wells with high dislocation densities
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10537355/
https://www.ncbi.nlm.nih.gov/pubmed/37764598
http://dx.doi.org/10.3390/nano13182569
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