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Determining the Number of Graphene Nanoribbons in Dual-Gate Field-Effect Transistors

[Image: see text] Bottom-up synthesized graphene nanoribbons (GNRs) are increasingly attracting interest due to their atomically controlled structure and customizable physical properties. In recent years, a range of GNR-based field-effect transistors (FETs) has been fabricated, with several demonstr...

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Autores principales: Zhang, Jian, Barin, Gabriela Borin, Furrer, Roman, Du, Cheng-Zhuo, Wang, Xiao-Ye, Müllen, Klaus, Ruffieux, Pascal, Fasel, Roman, Calame, Michel, Perrin, Mickael L.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10540264/
https://www.ncbi.nlm.nih.gov/pubmed/37671914
http://dx.doi.org/10.1021/acs.nanolett.3c01931
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author Zhang, Jian
Barin, Gabriela Borin
Furrer, Roman
Du, Cheng-Zhuo
Wang, Xiao-Ye
Müllen, Klaus
Ruffieux, Pascal
Fasel, Roman
Calame, Michel
Perrin, Mickael L.
author_facet Zhang, Jian
Barin, Gabriela Borin
Furrer, Roman
Du, Cheng-Zhuo
Wang, Xiao-Ye
Müllen, Klaus
Ruffieux, Pascal
Fasel, Roman
Calame, Michel
Perrin, Mickael L.
author_sort Zhang, Jian
collection PubMed
description [Image: see text] Bottom-up synthesized graphene nanoribbons (GNRs) are increasingly attracting interest due to their atomically controlled structure and customizable physical properties. In recent years, a range of GNR-based field-effect transistors (FETs) has been fabricated, with several demonstrating quantum-dot (QD) behavior at cryogenic temperatures. However, understanding the relationship between the cryogenic charge-transport characteristics and the number of the GNRs in the device is challenging, as the length and location of the GNRs in the junction are not precisely controlled. Here, we present a methodology based on a dual-gate FET that allows us to identify different scenarios, such as single GNRs, double or multiple GNRs in parallel, and a single GNR interacting with charge traps. Our dual-gate FET architecture therefore offers a quantitative approach for comprehending charge transport in atomically precise GNRs.
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spelling pubmed-105402642023-09-30 Determining the Number of Graphene Nanoribbons in Dual-Gate Field-Effect Transistors Zhang, Jian Barin, Gabriela Borin Furrer, Roman Du, Cheng-Zhuo Wang, Xiao-Ye Müllen, Klaus Ruffieux, Pascal Fasel, Roman Calame, Michel Perrin, Mickael L. Nano Lett [Image: see text] Bottom-up synthesized graphene nanoribbons (GNRs) are increasingly attracting interest due to their atomically controlled structure and customizable physical properties. In recent years, a range of GNR-based field-effect transistors (FETs) has been fabricated, with several demonstrating quantum-dot (QD) behavior at cryogenic temperatures. However, understanding the relationship between the cryogenic charge-transport characteristics and the number of the GNRs in the device is challenging, as the length and location of the GNRs in the junction are not precisely controlled. Here, we present a methodology based on a dual-gate FET that allows us to identify different scenarios, such as single GNRs, double or multiple GNRs in parallel, and a single GNR interacting with charge traps. Our dual-gate FET architecture therefore offers a quantitative approach for comprehending charge transport in atomically precise GNRs. American Chemical Society 2023-09-06 /pmc/articles/PMC10540264/ /pubmed/37671914 http://dx.doi.org/10.1021/acs.nanolett.3c01931 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Zhang, Jian
Barin, Gabriela Borin
Furrer, Roman
Du, Cheng-Zhuo
Wang, Xiao-Ye
Müllen, Klaus
Ruffieux, Pascal
Fasel, Roman
Calame, Michel
Perrin, Mickael L.
Determining the Number of Graphene Nanoribbons in Dual-Gate Field-Effect Transistors
title Determining the Number of Graphene Nanoribbons in Dual-Gate Field-Effect Transistors
title_full Determining the Number of Graphene Nanoribbons in Dual-Gate Field-Effect Transistors
title_fullStr Determining the Number of Graphene Nanoribbons in Dual-Gate Field-Effect Transistors
title_full_unstemmed Determining the Number of Graphene Nanoribbons in Dual-Gate Field-Effect Transistors
title_short Determining the Number of Graphene Nanoribbons in Dual-Gate Field-Effect Transistors
title_sort determining the number of graphene nanoribbons in dual-gate field-effect transistors
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10540264/
https://www.ncbi.nlm.nih.gov/pubmed/37671914
http://dx.doi.org/10.1021/acs.nanolett.3c01931
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