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Effect of the alumina micro-particle sizes on the thermal conductivity and dynamic mechanical property of epoxy resin

Epoxy thermal conductive adhesives with high thermal conductivity and dynamic mechanical properties are important thermally conductive materials for fabricating highly integrated electronic devices. In this paper, micro-Al(2)O(3) is used as a thermally conductive filler for the epoxy resin composite...

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Detalles Bibliográficos
Autores principales: Xu, Zhe, Zhang, Cheng, Li, Yang, Zou, Jun, Li, Yuefeng, Yang, Bobo, Hu, Rongrong, Qian, Qi
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Public Library of Science 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10575537/
https://www.ncbi.nlm.nih.gov/pubmed/37831678
http://dx.doi.org/10.1371/journal.pone.0292878
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author Xu, Zhe
Zhang, Cheng
Li, Yang
Zou, Jun
Li, Yuefeng
Yang, Bobo
Hu, Rongrong
Qian, Qi
author_facet Xu, Zhe
Zhang, Cheng
Li, Yang
Zou, Jun
Li, Yuefeng
Yang, Bobo
Hu, Rongrong
Qian, Qi
author_sort Xu, Zhe
collection PubMed
description Epoxy thermal conductive adhesives with high thermal conductivity and dynamic mechanical properties are important thermally conductive materials for fabricating highly integrated electronic devices. In this paper, micro-Al(2)O(3) is used as a thermally conductive filler for the epoxy resin composite and investigated the effect of micron-sized alumina particle size on the thermal conductivity and dynamic mechanical property of epoxy resin by the transient planar hot plate method and DMA (Dynamic mechanical analysis). The experimental results show that with the same amount of alumina filling, the thermal conductivity and Tg (glass transition temperature) of epoxy/Al(2)O(3) composite material decrease with the increase of alumina particle size. The maximum thermal conductivity of the composite material is 0.679 (W/mK), while the energy storage modulus of epoxy/Al(2)O(3) composite material increases with the increase of alumina particle size, and the maximum energy storage modulus of the composite material is 160MPa. Compared with pure epoxy resin, the thermal conductivity and energy storage modulus have increased by 2.7 and 3.2 times, respectively. The epoxy/Al(2)O(3) composite was applied to the COB (Chips On Board) type LED package, and the substrate temperature of the LED dropped to the lowest after 1.5 hours of operation using EP-A5 composite, and the temperature was stabilized at 38.2°C, indicating that the addition of 5-micron alumina composite has the best heat dissipation in the COB type LED package. These results are critical for the implementation of particulate-filled polymer composites in practical applications because relaxed material specifications and handling procedures can be incorporated in production environments to improve efficiency.
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spelling pubmed-105755372023-10-14 Effect of the alumina micro-particle sizes on the thermal conductivity and dynamic mechanical property of epoxy resin Xu, Zhe Zhang, Cheng Li, Yang Zou, Jun Li, Yuefeng Yang, Bobo Hu, Rongrong Qian, Qi PLoS One Research Article Epoxy thermal conductive adhesives with high thermal conductivity and dynamic mechanical properties are important thermally conductive materials for fabricating highly integrated electronic devices. In this paper, micro-Al(2)O(3) is used as a thermally conductive filler for the epoxy resin composite and investigated the effect of micron-sized alumina particle size on the thermal conductivity and dynamic mechanical property of epoxy resin by the transient planar hot plate method and DMA (Dynamic mechanical analysis). The experimental results show that with the same amount of alumina filling, the thermal conductivity and Tg (glass transition temperature) of epoxy/Al(2)O(3) composite material decrease with the increase of alumina particle size. The maximum thermal conductivity of the composite material is 0.679 (W/mK), while the energy storage modulus of epoxy/Al(2)O(3) composite material increases with the increase of alumina particle size, and the maximum energy storage modulus of the composite material is 160MPa. Compared with pure epoxy resin, the thermal conductivity and energy storage modulus have increased by 2.7 and 3.2 times, respectively. The epoxy/Al(2)O(3) composite was applied to the COB (Chips On Board) type LED package, and the substrate temperature of the LED dropped to the lowest after 1.5 hours of operation using EP-A5 composite, and the temperature was stabilized at 38.2°C, indicating that the addition of 5-micron alumina composite has the best heat dissipation in the COB type LED package. These results are critical for the implementation of particulate-filled polymer composites in practical applications because relaxed material specifications and handling procedures can be incorporated in production environments to improve efficiency. Public Library of Science 2023-10-13 /pmc/articles/PMC10575537/ /pubmed/37831678 http://dx.doi.org/10.1371/journal.pone.0292878 Text en © 2023 Xu et al https://creativecommons.org/licenses/by/4.0/This is an open access article distributed under the terms of the Creative Commons Attribution License (https://creativecommons.org/licenses/by/4.0/) , which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.
spellingShingle Research Article
Xu, Zhe
Zhang, Cheng
Li, Yang
Zou, Jun
Li, Yuefeng
Yang, Bobo
Hu, Rongrong
Qian, Qi
Effect of the alumina micro-particle sizes on the thermal conductivity and dynamic mechanical property of epoxy resin
title Effect of the alumina micro-particle sizes on the thermal conductivity and dynamic mechanical property of epoxy resin
title_full Effect of the alumina micro-particle sizes on the thermal conductivity and dynamic mechanical property of epoxy resin
title_fullStr Effect of the alumina micro-particle sizes on the thermal conductivity and dynamic mechanical property of epoxy resin
title_full_unstemmed Effect of the alumina micro-particle sizes on the thermal conductivity and dynamic mechanical property of epoxy resin
title_short Effect of the alumina micro-particle sizes on the thermal conductivity and dynamic mechanical property of epoxy resin
title_sort effect of the alumina micro-particle sizes on the thermal conductivity and dynamic mechanical property of epoxy resin
topic Research Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10575537/
https://www.ncbi.nlm.nih.gov/pubmed/37831678
http://dx.doi.org/10.1371/journal.pone.0292878
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