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Distinguishing Electronic and Vibronic Coherence in 2D Spectra by Their Temperature Dependence
[Image: see text] Long-lived oscillations in 2D spectra of chlorophylls are at the heart of an ongoing debate. Their physical origin is either a multipigment effect, such as excitonic coherence, or localized vibrations. We show how relative phase differences of diagonal- and cross-peak oscillations...
| Autores principales: | , , , |
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| Formato: | Online Artículo Texto |
| Lenguaje: | English |
| Publicado: |
American Chemical Society
2014
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| Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3917822/ https://www.ncbi.nlm.nih.gov/pubmed/24527180 http://dx.doi.org/10.1021/jz402468c |