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Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green
Strong localization effect in self-assembled InGaN quantum dots (QDs) grown by metalorganic chemical vapor deposition has been evidenced by temperature-dependent photoluminescence (PL) at different excitation power. The integrated emission intensity increases gradually in the range from 30 to 160 K...
Autores principales: | , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Springer US
2015
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4384949/ https://www.ncbi.nlm.nih.gov/pubmed/25852328 http://dx.doi.org/10.1186/s11671-015-0772-z |
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author | Weng, Guo-En Zhao, Wan-Ru Chen, Shao-Qiang Akiyama, Hidefumi Li, Zeng-Cheng Liu, Jian-Ping Zhang, Bao-Ping |
author_facet | Weng, Guo-En Zhao, Wan-Ru Chen, Shao-Qiang Akiyama, Hidefumi Li, Zeng-Cheng Liu, Jian-Ping Zhang, Bao-Ping |
author_sort | Weng, Guo-En |
collection | PubMed |
description | Strong localization effect in self-assembled InGaN quantum dots (QDs) grown by metalorganic chemical vapor deposition has been evidenced by temperature-dependent photoluminescence (PL) at different excitation power. The integrated emission intensity increases gradually in the range from 30 to 160 K and then decreases with a further increase in temperature at high excitation intensity, while this phenomenon disappeared at low excitation intensity. Under high excitation, about 40% emission enhancement at 160 K compared to that at low temperature, as well as a higher internal quantum efficiency (IQE) of 41.1%, was observed. A strong localization model is proposed to describe the possible processes of carrier transport, relaxation, and recombination. Using this model, the evolution of excitation-power-dependent emission intensity, shift of peak energy, and linewidth variation with elevating temperature is well explained. Finally, two-component decays of time-resolved PL (TRPL) with various excitation intensities are observed and analyzed with the biexponential model, which enables us to further understand the carrier relaxation dynamics in the InGaN QDs. |
format | Online Article Text |
id | pubmed-4384949 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2015 |
publisher | Springer US |
record_format | MEDLINE/PubMed |
spelling | pubmed-43849492015-04-07 Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green Weng, Guo-En Zhao, Wan-Ru Chen, Shao-Qiang Akiyama, Hidefumi Li, Zeng-Cheng Liu, Jian-Ping Zhang, Bao-Ping Nanoscale Res Lett Nano Express Strong localization effect in self-assembled InGaN quantum dots (QDs) grown by metalorganic chemical vapor deposition has been evidenced by temperature-dependent photoluminescence (PL) at different excitation power. The integrated emission intensity increases gradually in the range from 30 to 160 K and then decreases with a further increase in temperature at high excitation intensity, while this phenomenon disappeared at low excitation intensity. Under high excitation, about 40% emission enhancement at 160 K compared to that at low temperature, as well as a higher internal quantum efficiency (IQE) of 41.1%, was observed. A strong localization model is proposed to describe the possible processes of carrier transport, relaxation, and recombination. Using this model, the evolution of excitation-power-dependent emission intensity, shift of peak energy, and linewidth variation with elevating temperature is well explained. Finally, two-component decays of time-resolved PL (TRPL) with various excitation intensities are observed and analyzed with the biexponential model, which enables us to further understand the carrier relaxation dynamics in the InGaN QDs. Springer US 2015-02-03 /pmc/articles/PMC4384949/ /pubmed/25852328 http://dx.doi.org/10.1186/s11671-015-0772-z Text en © Weng et al.; licensee Springer. 2015 This is an Open Access article distributed under the terms of the Creative Commons Attribution License (http://creativecommons.org/licenses/by/4.0), which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly credited. |
spellingShingle | Nano Express Weng, Guo-En Zhao, Wan-Ru Chen, Shao-Qiang Akiyama, Hidefumi Li, Zeng-Cheng Liu, Jian-Ping Zhang, Bao-Ping Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green |
title | Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green |
title_full | Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green |
title_fullStr | Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green |
title_full_unstemmed | Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green |
title_short | Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green |
title_sort | strong localization effect and carrier relaxation dynamics in self-assembled ingan quantum dots emitting in the green |
topic | Nano Express |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4384949/ https://www.ncbi.nlm.nih.gov/pubmed/25852328 http://dx.doi.org/10.1186/s11671-015-0772-z |
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