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Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green

Strong localization effect in self-assembled InGaN quantum dots (QDs) grown by metalorganic chemical vapor deposition has been evidenced by temperature-dependent photoluminescence (PL) at different excitation power. The integrated emission intensity increases gradually in the range from 30 to 160 K...

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Autores principales: Weng, Guo-En, Zhao, Wan-Ru, Chen, Shao-Qiang, Akiyama, Hidefumi, Li, Zeng-Cheng, Liu, Jian-Ping, Zhang, Bao-Ping
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Springer US 2015
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4384949/
https://www.ncbi.nlm.nih.gov/pubmed/25852328
http://dx.doi.org/10.1186/s11671-015-0772-z
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author Weng, Guo-En
Zhao, Wan-Ru
Chen, Shao-Qiang
Akiyama, Hidefumi
Li, Zeng-Cheng
Liu, Jian-Ping
Zhang, Bao-Ping
author_facet Weng, Guo-En
Zhao, Wan-Ru
Chen, Shao-Qiang
Akiyama, Hidefumi
Li, Zeng-Cheng
Liu, Jian-Ping
Zhang, Bao-Ping
author_sort Weng, Guo-En
collection PubMed
description Strong localization effect in self-assembled InGaN quantum dots (QDs) grown by metalorganic chemical vapor deposition has been evidenced by temperature-dependent photoluminescence (PL) at different excitation power. The integrated emission intensity increases gradually in the range from 30 to 160 K and then decreases with a further increase in temperature at high excitation intensity, while this phenomenon disappeared at low excitation intensity. Under high excitation, about 40% emission enhancement at 160 K compared to that at low temperature, as well as a higher internal quantum efficiency (IQE) of 41.1%, was observed. A strong localization model is proposed to describe the possible processes of carrier transport, relaxation, and recombination. Using this model, the evolution of excitation-power-dependent emission intensity, shift of peak energy, and linewidth variation with elevating temperature is well explained. Finally, two-component decays of time-resolved PL (TRPL) with various excitation intensities are observed and analyzed with the biexponential model, which enables us to further understand the carrier relaxation dynamics in the InGaN QDs.
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spelling pubmed-43849492015-04-07 Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green Weng, Guo-En Zhao, Wan-Ru Chen, Shao-Qiang Akiyama, Hidefumi Li, Zeng-Cheng Liu, Jian-Ping Zhang, Bao-Ping Nanoscale Res Lett Nano Express Strong localization effect in self-assembled InGaN quantum dots (QDs) grown by metalorganic chemical vapor deposition has been evidenced by temperature-dependent photoluminescence (PL) at different excitation power. The integrated emission intensity increases gradually in the range from 30 to 160 K and then decreases with a further increase in temperature at high excitation intensity, while this phenomenon disappeared at low excitation intensity. Under high excitation, about 40% emission enhancement at 160 K compared to that at low temperature, as well as a higher internal quantum efficiency (IQE) of 41.1%, was observed. A strong localization model is proposed to describe the possible processes of carrier transport, relaxation, and recombination. Using this model, the evolution of excitation-power-dependent emission intensity, shift of peak energy, and linewidth variation with elevating temperature is well explained. Finally, two-component decays of time-resolved PL (TRPL) with various excitation intensities are observed and analyzed with the biexponential model, which enables us to further understand the carrier relaxation dynamics in the InGaN QDs. Springer US 2015-02-03 /pmc/articles/PMC4384949/ /pubmed/25852328 http://dx.doi.org/10.1186/s11671-015-0772-z Text en © Weng et al.; licensee Springer. 2015 This is an Open Access article distributed under the terms of the Creative Commons Attribution License (http://creativecommons.org/licenses/by/4.0), which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly credited.
spellingShingle Nano Express
Weng, Guo-En
Zhao, Wan-Ru
Chen, Shao-Qiang
Akiyama, Hidefumi
Li, Zeng-Cheng
Liu, Jian-Ping
Zhang, Bao-Ping
Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green
title Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green
title_full Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green
title_fullStr Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green
title_full_unstemmed Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green
title_short Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green
title_sort strong localization effect and carrier relaxation dynamics in self-assembled ingan quantum dots emitting in the green
topic Nano Express
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4384949/
https://www.ncbi.nlm.nih.gov/pubmed/25852328
http://dx.doi.org/10.1186/s11671-015-0772-z
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