Strong frequency dependence of vibrational relaxation in bulk and surface water reveals sub-picosecond structural heterogeneity

Because of strong hydrogen bonding in liquid water, intermolecular interactions between water molecules are highly delocalized. Previous two-dimensional infrared spectroscopy experiments have indicated that this delocalization smears out the structural heterogeneity of neat H(2)O. Here we report on...

Descripción completa

Detalles Bibliográficos
Autores principales: van der Post, Sietse T., Hsieh, Cho-Shuen, Okuno, Masanari, Nagata, Yuki, Bakker, Huib J., Bonn, Mischa, Hunger, Johannes
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Pub. Group 2015
Materias:
Article
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4595750/
https://www.ncbi.nlm.nih.gov/pubmed/26382651
http://dx.doi.org/10.1038/ncomms9384

Internet

https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4595750/
https://www.ncbi.nlm.nih.gov/pubmed/26382651
http://dx.doi.org/10.1038/ncomms9384

Ejemplares similares