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Strong frequency dependence of vibrational relaxation in bulk and surface water reveals sub-picosecond structural heterogeneity

Because of strong hydrogen bonding in liquid water, intermolecular interactions between water molecules are highly delocalized. Previous two-dimensional infrared spectroscopy experiments have indicated that this delocalization smears out the structural heterogeneity of neat H(2)O. Here we report on...

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Detalles Bibliográficos
Autores principales:	van der Post, Sietse T., Hsieh, Cho-Shuen, Okuno, Masanari, Nagata, Yuki, Bakker, Huib J., Bonn, Mischa, Hunger, Johannes
Formato:	Online Artículo Texto
Lenguaje:	English
Publicado:	Nature Pub. Group 2015
Materias:	Article
Acceso en línea:	https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4595750/ https://www.ncbi.nlm.nih.gov/pubmed/26382651 http://dx.doi.org/10.1038/ncomms9384

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