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Rational design of carbon nitride photocatalysts by identification of cyanamide defects as catalytically relevant sites

The heptazine-based polymer melon (also known as graphitic carbon nitride, g-C(3)N(4)) is a promising photocatalyst for hydrogen evolution. Nonetheless, attempts to improve its inherently low activity are rarely based on rational approaches because of a lack of fundamental understanding of its mecha...

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Detalles Bibliográficos
Autores principales: Lau, Vincent Wing-hei, Moudrakovski, Igor, Botari, Tiago, Weinberger, Simon, Mesch, Maria B., Duppel, Viola, Senker, Jürgen, Blum, Volker, Lotsch, Bettina V.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4941108/
https://www.ncbi.nlm.nih.gov/pubmed/27387536
http://dx.doi.org/10.1038/ncomms12165