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The Role of Rydberg–Valence Coupling in the Ultrafast Relaxation Dynamics of Acetone
[Image: see text] The electronic structure of excited states of acetone is represented by a Rydberg manifold that is coupled to valence states which provide very fast and efficient relaxation pathways. We observe and characterize the transfer of population from photoexcited Rydberg states (6p, 6d, 7...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical
Society
2017
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5608382/ https://www.ncbi.nlm.nih.gov/pubmed/28737942 http://dx.doi.org/10.1021/acs.jpca.7b05012 |