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Highly selective nickel-catalyzed gem-difluoropropargylation of unactivated alkylzinc reagents
In spite of the important applications of difluoroalkylated molecules in medicinal chemistry, to date, the reaction of difluoroalkylating reagents with unactivated, aliphatic substrates through a controllable manner remains challenging and has not been reported. Here we describe an efficient nickel-...
Autores principales: | , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2017
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5684216/ https://www.ncbi.nlm.nih.gov/pubmed/29133781 http://dx.doi.org/10.1038/s41467-017-01540-1 |
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author | An, Lun Xu, Chang Zhang, Xingang |
author_facet | An, Lun Xu, Chang Zhang, Xingang |
author_sort | An, Lun |
collection | PubMed |
description | In spite of the important applications of difluoroalkylated molecules in medicinal chemistry, to date, the reaction of difluoroalkylating reagents with unactivated, aliphatic substrates through a controllable manner remains challenging and has not been reported. Here we describe an efficient nickel-catalyzed cross-coupling of unactivated alkylzinc reagen\ts with gem-difluoropropargyl bromides. The reaction proceeds under mild reaction conditions with high efficiency and excellent regiochemical selectivity. Transformations of the resulting difluoroalkylated alkanes lead to a variety of biologically active molecules, providing a facile route for applications in drug discovery and development. Preliminary mechanistic studies reveal that an alkyl nickel intermediate [Ni(tpy)alkyl] (tpy, terpyridine) is involved in the catalytic cycle. |
format | Online Article Text |
id | pubmed-5684216 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2017 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-56842162017-11-17 Highly selective nickel-catalyzed gem-difluoropropargylation of unactivated alkylzinc reagents An, Lun Xu, Chang Zhang, Xingang Nat Commun Article In spite of the important applications of difluoroalkylated molecules in medicinal chemistry, to date, the reaction of difluoroalkylating reagents with unactivated, aliphatic substrates through a controllable manner remains challenging and has not been reported. Here we describe an efficient nickel-catalyzed cross-coupling of unactivated alkylzinc reagen\ts with gem-difluoropropargyl bromides. The reaction proceeds under mild reaction conditions with high efficiency and excellent regiochemical selectivity. Transformations of the resulting difluoroalkylated alkanes lead to a variety of biologically active molecules, providing a facile route for applications in drug discovery and development. Preliminary mechanistic studies reveal that an alkyl nickel intermediate [Ni(tpy)alkyl] (tpy, terpyridine) is involved in the catalytic cycle. Nature Publishing Group UK 2017-11-13 /pmc/articles/PMC5684216/ /pubmed/29133781 http://dx.doi.org/10.1038/s41467-017-01540-1 Text en © The Author(s) 2017 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article An, Lun Xu, Chang Zhang, Xingang Highly selective nickel-catalyzed gem-difluoropropargylation of unactivated alkylzinc reagents |
title | Highly selective nickel-catalyzed gem-difluoropropargylation of unactivated alkylzinc reagents |
title_full | Highly selective nickel-catalyzed gem-difluoropropargylation of unactivated alkylzinc reagents |
title_fullStr | Highly selective nickel-catalyzed gem-difluoropropargylation of unactivated alkylzinc reagents |
title_full_unstemmed | Highly selective nickel-catalyzed gem-difluoropropargylation of unactivated alkylzinc reagents |
title_short | Highly selective nickel-catalyzed gem-difluoropropargylation of unactivated alkylzinc reagents |
title_sort | highly selective nickel-catalyzed gem-difluoropropargylation of unactivated alkylzinc reagents |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5684216/ https://www.ncbi.nlm.nih.gov/pubmed/29133781 http://dx.doi.org/10.1038/s41467-017-01540-1 |
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