Cargando…

Direct Auger recombination and density-dependent hole diffusion in InN

Indium nitride has a good potential for infrared optoelectronics, yet it suffers from fast nonradiative recombination, the true origin of which has not been established with certainty. The diffusion length of free carriers at high densities is not well investigated either. Here, we study carrier rec...

Descripción completa

Detalles Bibliográficos
Autores principales: Aleksiejūnas, Ramūnas, Podlipskas, Žydrūnas, Nargelas, Saulius, Kadys, Arūnas, Kolenda, Marek, Nomeika, Kazimieras, Mickevičius, Jūras, Tamulaitis, Gintautas
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5854707/
https://www.ncbi.nlm.nih.gov/pubmed/29545555
http://dx.doi.org/10.1038/s41598-018-22832-6
_version_ 1783306958734884864
author Aleksiejūnas, Ramūnas
Podlipskas, Žydrūnas
Nargelas, Saulius
Kadys, Arūnas
Kolenda, Marek
Nomeika, Kazimieras
Mickevičius, Jūras
Tamulaitis, Gintautas
author_facet Aleksiejūnas, Ramūnas
Podlipskas, Žydrūnas
Nargelas, Saulius
Kadys, Arūnas
Kolenda, Marek
Nomeika, Kazimieras
Mickevičius, Jūras
Tamulaitis, Gintautas
author_sort Aleksiejūnas, Ramūnas
collection PubMed
description Indium nitride has a good potential for infrared optoelectronics, yet it suffers from fast nonradiative recombination, the true origin of which has not been established with certainty. The diffusion length of free carriers at high densities is not well investigated either. Here, we study carrier recombination and diffusion using the light-induced transient grating technique in InN epilayers grown by pulsed MOCVD on c-plane sapphire. We show that direct Auger recombination governs the lifetime of carriers at densities above ~10(18) cm(−3). The measured Auger recombination coefficient is (8 ± 1) × 10(−29) cm(−3). At carrier densities above ~5 × 10(19) cm(−3), we observe the saturation of Auger recombination rate due to phase space filling. The diffusion coefficient of holes scales linearly with carrier density, increasing from 1 cm(2)/s in low-doped layers at low excitations and up to ~40 cm(2)/s at highest carrier densities. The resulting carrier diffusion length remains within 100–300 nm range, which is comparable to the light absorption depth. This feature is required for efficient carrier extraction in bipolar devices, thus suggesting MOCVD-grown InN as the material fit for photovoltaic and photonic applications.
format Online
Article
Text
id pubmed-5854707
institution National Center for Biotechnology Information
language English
publishDate 2018
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-58547072018-03-22 Direct Auger recombination and density-dependent hole diffusion in InN Aleksiejūnas, Ramūnas Podlipskas, Žydrūnas Nargelas, Saulius Kadys, Arūnas Kolenda, Marek Nomeika, Kazimieras Mickevičius, Jūras Tamulaitis, Gintautas Sci Rep Article Indium nitride has a good potential for infrared optoelectronics, yet it suffers from fast nonradiative recombination, the true origin of which has not been established with certainty. The diffusion length of free carriers at high densities is not well investigated either. Here, we study carrier recombination and diffusion using the light-induced transient grating technique in InN epilayers grown by pulsed MOCVD on c-plane sapphire. We show that direct Auger recombination governs the lifetime of carriers at densities above ~10(18) cm(−3). The measured Auger recombination coefficient is (8 ± 1) × 10(−29) cm(−3). At carrier densities above ~5 × 10(19) cm(−3), we observe the saturation of Auger recombination rate due to phase space filling. The diffusion coefficient of holes scales linearly with carrier density, increasing from 1 cm(2)/s in low-doped layers at low excitations and up to ~40 cm(2)/s at highest carrier densities. The resulting carrier diffusion length remains within 100–300 nm range, which is comparable to the light absorption depth. This feature is required for efficient carrier extraction in bipolar devices, thus suggesting MOCVD-grown InN as the material fit for photovoltaic and photonic applications. Nature Publishing Group UK 2018-03-15 /pmc/articles/PMC5854707/ /pubmed/29545555 http://dx.doi.org/10.1038/s41598-018-22832-6 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Aleksiejūnas, Ramūnas
Podlipskas, Žydrūnas
Nargelas, Saulius
Kadys, Arūnas
Kolenda, Marek
Nomeika, Kazimieras
Mickevičius, Jūras
Tamulaitis, Gintautas
Direct Auger recombination and density-dependent hole diffusion in InN
title Direct Auger recombination and density-dependent hole diffusion in InN
title_full Direct Auger recombination and density-dependent hole diffusion in InN
title_fullStr Direct Auger recombination and density-dependent hole diffusion in InN
title_full_unstemmed Direct Auger recombination and density-dependent hole diffusion in InN
title_short Direct Auger recombination and density-dependent hole diffusion in InN
title_sort direct auger recombination and density-dependent hole diffusion in inn
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5854707/
https://www.ncbi.nlm.nih.gov/pubmed/29545555
http://dx.doi.org/10.1038/s41598-018-22832-6
work_keys_str_mv AT aleksiejunasramunas directaugerrecombinationanddensitydependentholediffusionininn
AT podlipskaszydrunas directaugerrecombinationanddensitydependentholediffusionininn
AT nargelassaulius directaugerrecombinationanddensitydependentholediffusionininn
AT kadysarunas directaugerrecombinationanddensitydependentholediffusionininn
AT kolendamarek directaugerrecombinationanddensitydependentholediffusionininn
AT nomeikakazimieras directaugerrecombinationanddensitydependentholediffusionininn
AT mickeviciusjuras directaugerrecombinationanddensitydependentholediffusionininn
AT tamulaitisgintautas directaugerrecombinationanddensitydependentholediffusionininn