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Local protein solvation drives direct down-conversion in phycobiliprotein PC645 via incoherent vibronic transport
The mechanisms controlling excitation energy transport (EET) in light-harvesting complexes remain controversial. Following the observation of long-lived beats in 2D electronic spectroscopy of PC645, vibronic coherence, the delocalization of excited states between pigments supported by a resonant vib...
Autores principales: | Blau, Samuel M., Bennett, Doran I. G., Kreisbeck, Christoph, Scholes, Gregory D., Aspuru-Guzik, Alán |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
National Academy of Sciences
2018
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5899487/ https://www.ncbi.nlm.nih.gov/pubmed/29588417 http://dx.doi.org/10.1073/pnas.1800370115 |
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