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Heterogeneous Fe(3) single-cluster catalyst for ammonia synthesis via an associative mechanism

The current industrial ammonia synthesis relies on Haber–Bosch process that is initiated by the dissociative mechanism, in which the adsorbed N(2) dissociates directly, and thus is limited by Brønsted–Evans–Polanyi (BEP) relation. Here we propose a new strategy that an anchored Fe(3) cluster on the...

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Detalles Bibliográficos
Autores principales:	Liu, Jin-Cheng, Ma, Xue-Lu, Li, Yong, Wang, Yang-Gang, Xiao, Hai, Li, Jun
Formato:	Online Artículo Texto
Lenguaje:	English
Publicado:	Nature Publishing Group UK 2018
Materias:	Article
Acceso en línea:	https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5913218/ https://www.ncbi.nlm.nih.gov/pubmed/29686395 http://dx.doi.org/10.1038/s41467-018-03795-8

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