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Electron Information in Single- and Dual-Frequency Capacitive Discharges at Atmospheric Pressure

Determining the electron properties of weakly ionized gases, particularly in a high electron-neutral collisional condition, is a nontrivial task; thus, the mechanisms underlying the electron characteristics and electron heating structure in radio-frequency (rf) collisional discharges remain unclear....

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Autores principales: Park, Sanghoo, Choe, Wonho, Moon, Se Youn, Shi, Jian Jun
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5951922/
https://www.ncbi.nlm.nih.gov/pubmed/29760408
http://dx.doi.org/10.1038/s41598-018-25892-w
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author Park, Sanghoo
Choe, Wonho
Moon, Se Youn
Shi, Jian Jun
author_facet Park, Sanghoo
Choe, Wonho
Moon, Se Youn
Shi, Jian Jun
author_sort Park, Sanghoo
collection PubMed
description Determining the electron properties of weakly ionized gases, particularly in a high electron-neutral collisional condition, is a nontrivial task; thus, the mechanisms underlying the electron characteristics and electron heating structure in radio-frequency (rf) collisional discharges remain unclear. Here, we report the electrical characteristics and electron information in single-frequency (4.52 MHz and 13.56 MHz) and dual-frequency (a combination of 4.52 MHz and 13.56 MHz) capacitive discharges within the abnormal α-mode regime at atmospheric pressure. A continuum radiation-based electron diagnostic method is employed to estimate the electron density (n(e)) and temperature (T(e)). Our experimental observations reveal that time-averaged n(e) (7.7–14 × 10(11) cm(−3)) and T(e) (1.75–2.5 eV) can be independently controlled in dual-frequency discharge, whereas such control is nontrivial in single-frequency discharge, which shows a linear increase in n(e) and little to no change in T(e) with increases in the rf input power. Furthermore, the two-dimensional spatiotemporal evolution of neutral bremsstrahlung and associated electron heating structures is demonstrated. These results reveal that a symmetric structure in electron heating becomes asymmetric (via a local suppression of electron temperature) as two-frequency power is simultaneously introduced.
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spelling pubmed-59519222018-05-21 Electron Information in Single- and Dual-Frequency Capacitive Discharges at Atmospheric Pressure Park, Sanghoo Choe, Wonho Moon, Se Youn Shi, Jian Jun Sci Rep Article Determining the electron properties of weakly ionized gases, particularly in a high electron-neutral collisional condition, is a nontrivial task; thus, the mechanisms underlying the electron characteristics and electron heating structure in radio-frequency (rf) collisional discharges remain unclear. Here, we report the electrical characteristics and electron information in single-frequency (4.52 MHz and 13.56 MHz) and dual-frequency (a combination of 4.52 MHz and 13.56 MHz) capacitive discharges within the abnormal α-mode regime at atmospheric pressure. A continuum radiation-based electron diagnostic method is employed to estimate the electron density (n(e)) and temperature (T(e)). Our experimental observations reveal that time-averaged n(e) (7.7–14 × 10(11) cm(−3)) and T(e) (1.75–2.5 eV) can be independently controlled in dual-frequency discharge, whereas such control is nontrivial in single-frequency discharge, which shows a linear increase in n(e) and little to no change in T(e) with increases in the rf input power. Furthermore, the two-dimensional spatiotemporal evolution of neutral bremsstrahlung and associated electron heating structures is demonstrated. These results reveal that a symmetric structure in electron heating becomes asymmetric (via a local suppression of electron temperature) as two-frequency power is simultaneously introduced. Nature Publishing Group UK 2018-05-14 /pmc/articles/PMC5951922/ /pubmed/29760408 http://dx.doi.org/10.1038/s41598-018-25892-w Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Park, Sanghoo
Choe, Wonho
Moon, Se Youn
Shi, Jian Jun
Electron Information in Single- and Dual-Frequency Capacitive Discharges at Atmospheric Pressure
title Electron Information in Single- and Dual-Frequency Capacitive Discharges at Atmospheric Pressure
title_full Electron Information in Single- and Dual-Frequency Capacitive Discharges at Atmospheric Pressure
title_fullStr Electron Information in Single- and Dual-Frequency Capacitive Discharges at Atmospheric Pressure
title_full_unstemmed Electron Information in Single- and Dual-Frequency Capacitive Discharges at Atmospheric Pressure
title_short Electron Information in Single- and Dual-Frequency Capacitive Discharges at Atmospheric Pressure
title_sort electron information in single- and dual-frequency capacitive discharges at atmospheric pressure
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5951922/
https://www.ncbi.nlm.nih.gov/pubmed/29760408
http://dx.doi.org/10.1038/s41598-018-25892-w
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