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pH effects on the electrochemical reduction of CO((2)) towards C(2) products on stepped copper
We present a microkinetic model for CO((2)) reduction (CO((2))R) on Cu(211) towards C(2) products, based on energetics estimated from an explicit solvent model. We show that the differences in both Tafel slopes and pH dependence for C(1) vs C(2) activity arise from differences in their multi-step me...
Autores principales: | , , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2019
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6318338/ https://www.ncbi.nlm.nih.gov/pubmed/30604776 http://dx.doi.org/10.1038/s41467-018-07970-9 |