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Monitoring of Nonadiabatic Effects in Individual Chromophores by Femtosecond Double-Pump Single-Molecule Spectroscopy: A Model Study

We explore, by theoretical modeling and computer simulations, how nonadiabatic couplings of excited electronic states of a polyatomic chromophore manifest themselves in single-molecule signals on femtosecond timescales. The chromophore is modeled as a system with three electronic states (the ground...

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Detalles Bibliográficos
Autores principales: Gelin, Maxim F., Palacino-González, Elisa, Chen, Lipeng, Domcke, Wolfgang
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6359062/
https://www.ncbi.nlm.nih.gov/pubmed/30634541
http://dx.doi.org/10.3390/molecules24020231