Cargando…
Electrically Robust Single‐Crystalline WTe(2) Nanobelts for Nanoscale Electrical Interconnects
As the elements of integrated circuits are downsized to the nanoscale, the current Cu‐based interconnects are facing limitations due to increased resistivity and decreased current‐carrying capacity because of scaling. Here, the bottom‐up synthesis of single‐crystalline WTe(2) nanobelts and low‐ and...
Autores principales: | , , , , , , , , , , , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
John Wiley and Sons Inc.
2018
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6364501/ https://www.ncbi.nlm.nih.gov/pubmed/30775229 http://dx.doi.org/10.1002/advs.201801370 |
_version_ | 1783393293266059264 |
---|---|
author | Song, Seunguk Kim, Se‐Yang Kwak, Jinsung Jo, Yongsu Kim, Jung Hwa Lee, Jong Hwa Lee, Jae‐Ung Kim, Jong Uk Yun, Hyung Duk Sim, Yeoseon Wang, Jaewon Lee, Do Hee Seok, Shi‐Hyun Kim, Tae‐il Cheong, Hyeonsik Lee, Zonghoon Kwon, Soon‐Yong |
author_facet | Song, Seunguk Kim, Se‐Yang Kwak, Jinsung Jo, Yongsu Kim, Jung Hwa Lee, Jong Hwa Lee, Jae‐Ung Kim, Jong Uk Yun, Hyung Duk Sim, Yeoseon Wang, Jaewon Lee, Do Hee Seok, Shi‐Hyun Kim, Tae‐il Cheong, Hyeonsik Lee, Zonghoon Kwon, Soon‐Yong |
author_sort | Song, Seunguk |
collection | PubMed |
description | As the elements of integrated circuits are downsized to the nanoscale, the current Cu‐based interconnects are facing limitations due to increased resistivity and decreased current‐carrying capacity because of scaling. Here, the bottom‐up synthesis of single‐crystalline WTe(2) nanobelts and low‐ and high‐field electrical characterization of nanoscale interconnect test structures in various ambient conditions are reported. Unlike exfoliated flakes obtained by the top‐down approach, the bottom‐up growth mode of WTe(2) nanobelts allows systemic characterization of the electrical properties of WTe(2) single crystals as a function of channel dimensions. Using a 1D heat transport model and a power law, it is determined that the breakdown of WTe(2) devices under vacuum and with AlO(x) capping layer follows an ideal pattern for Joule heating, far from edge scattering. High‐field electrical measurements and self‐heating modeling demonstrate that the WTe(2) nanobelts have a breakdown current density approaching ≈100 MA cm(−2), remarkably higher than those of conventional metals and other transition‐metal chalcogenides, and sustain the highest electrical power per channel length (≈16.4 W cm(−1)) among the interconnect candidates. The results suggest superior robustness of WTe(2) against high‐bias sweep and its possible applicability in future nanoelectronics. |
format | Online Article Text |
id | pubmed-6364501 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2018 |
publisher | John Wiley and Sons Inc. |
record_format | MEDLINE/PubMed |
spelling | pubmed-63645012019-02-15 Electrically Robust Single‐Crystalline WTe(2) Nanobelts for Nanoscale Electrical Interconnects Song, Seunguk Kim, Se‐Yang Kwak, Jinsung Jo, Yongsu Kim, Jung Hwa Lee, Jong Hwa Lee, Jae‐Ung Kim, Jong Uk Yun, Hyung Duk Sim, Yeoseon Wang, Jaewon Lee, Do Hee Seok, Shi‐Hyun Kim, Tae‐il Cheong, Hyeonsik Lee, Zonghoon Kwon, Soon‐Yong Adv Sci (Weinh) Full Papers As the elements of integrated circuits are downsized to the nanoscale, the current Cu‐based interconnects are facing limitations due to increased resistivity and decreased current‐carrying capacity because of scaling. Here, the bottom‐up synthesis of single‐crystalline WTe(2) nanobelts and low‐ and high‐field electrical characterization of nanoscale interconnect test structures in various ambient conditions are reported. Unlike exfoliated flakes obtained by the top‐down approach, the bottom‐up growth mode of WTe(2) nanobelts allows systemic characterization of the electrical properties of WTe(2) single crystals as a function of channel dimensions. Using a 1D heat transport model and a power law, it is determined that the breakdown of WTe(2) devices under vacuum and with AlO(x) capping layer follows an ideal pattern for Joule heating, far from edge scattering. High‐field electrical measurements and self‐heating modeling demonstrate that the WTe(2) nanobelts have a breakdown current density approaching ≈100 MA cm(−2), remarkably higher than those of conventional metals and other transition‐metal chalcogenides, and sustain the highest electrical power per channel length (≈16.4 W cm(−1)) among the interconnect candidates. The results suggest superior robustness of WTe(2) against high‐bias sweep and its possible applicability in future nanoelectronics. John Wiley and Sons Inc. 2018-12-12 /pmc/articles/PMC6364501/ /pubmed/30775229 http://dx.doi.org/10.1002/advs.201801370 Text en © 2018 The Authors. Published by WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim This is an open access article under the terms of the http://creativecommons.org/licenses/by/4.0/ License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited. |
spellingShingle | Full Papers Song, Seunguk Kim, Se‐Yang Kwak, Jinsung Jo, Yongsu Kim, Jung Hwa Lee, Jong Hwa Lee, Jae‐Ung Kim, Jong Uk Yun, Hyung Duk Sim, Yeoseon Wang, Jaewon Lee, Do Hee Seok, Shi‐Hyun Kim, Tae‐il Cheong, Hyeonsik Lee, Zonghoon Kwon, Soon‐Yong Electrically Robust Single‐Crystalline WTe(2) Nanobelts for Nanoscale Electrical Interconnects |
title | Electrically Robust Single‐Crystalline WTe(2) Nanobelts for Nanoscale Electrical Interconnects |
title_full | Electrically Robust Single‐Crystalline WTe(2) Nanobelts for Nanoscale Electrical Interconnects |
title_fullStr | Electrically Robust Single‐Crystalline WTe(2) Nanobelts for Nanoscale Electrical Interconnects |
title_full_unstemmed | Electrically Robust Single‐Crystalline WTe(2) Nanobelts for Nanoscale Electrical Interconnects |
title_short | Electrically Robust Single‐Crystalline WTe(2) Nanobelts for Nanoscale Electrical Interconnects |
title_sort | electrically robust single‐crystalline wte(2) nanobelts for nanoscale electrical interconnects |
topic | Full Papers |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6364501/ https://www.ncbi.nlm.nih.gov/pubmed/30775229 http://dx.doi.org/10.1002/advs.201801370 |
work_keys_str_mv | AT songseunguk electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT kimseyang electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT kwakjinsung electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT joyongsu electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT kimjunghwa electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT leejonghwa electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT leejaeung electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT kimjonguk electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT yunhyungduk electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT simyeoseon electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT wangjaewon electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT leedohee electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT seokshihyun electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT kimtaeil electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT cheonghyeonsik electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT leezonghoon electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects AT kwonsoonyong electricallyrobustsinglecrystallinewte2nanobeltsfornanoscaleelectricalinterconnects |