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Mechanism unravelling for ultrafast and selective (99)TcO(4)(–) uptake by a radiation-resistant cationic covalent organic framework: a combined radiological experiment and molecular dynamics simulation study
(99)Tc is one of the most problematic fission products in the nuclear fuel cycle owing to its large inventory in used nuclear fuel, long half-life, potential radiation hazard, high environmental mobility of its major species (99)TcO(4)(–), and its redox-active nature. Ideally, (99)TcO(4)(–) should b...
Autores principales: | , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Royal Society of Chemistry
2019
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6471554/ https://www.ncbi.nlm.nih.gov/pubmed/31057756 http://dx.doi.org/10.1039/c9sc00172g |