Cargando…

A New Analytic Formula for Minority Carrier Decay Length Extraction from Scanning Photocurrent Profiles in Ohmic-Contact Nanowire Devices

Spatially resolved current measurements such as scanning photocurrent microscopy (SPCM) have been extensively applied to investigate carrier transport properties in semiconductor nanowires. A traditional simple-exponential-decay formula based on the assumption of carrier diffusion dominance in the s...

Descripción completa

Detalles Bibliográficos
Autores principales: Chu, Cheng-Hao, Mao, Ming-Hua, Yang, Che-Wei, Lin, Hao-Hsiung
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6603194/
https://www.ncbi.nlm.nih.gov/pubmed/31263209
http://dx.doi.org/10.1038/s41598-019-46020-2
_version_ 1783431470027636736
author Chu, Cheng-Hao
Mao, Ming-Hua
Yang, Che-Wei
Lin, Hao-Hsiung
author_facet Chu, Cheng-Hao
Mao, Ming-Hua
Yang, Che-Wei
Lin, Hao-Hsiung
author_sort Chu, Cheng-Hao
collection PubMed
description Spatially resolved current measurements such as scanning photocurrent microscopy (SPCM) have been extensively applied to investigate carrier transport properties in semiconductor nanowires. A traditional simple-exponential-decay formula based on the assumption of carrier diffusion dominance in the scanning photocurrent profiles can be applied for carrier diffusion length extraction using SPCM in Schottky-contact-based or p-n junction-based devices where large built-in electric fields exist. However, it is also important to study the electric-field dependent transport properties in widely used ohmic-contact nanowire devices where the assumption of carrier diffusion dominance is invalid. Here we derive an analytic formula for scanning photocurrent profiles in such ohmic-contact nanowire devices under uniform applied electric fields and weak optical excitation. Under these operation conditions and the influence of photo-carrier-induced electric field, the scanning photocurrent profile and the carrier spatial distribution strikingly do not share the same functional form. Instead, a surprising new analytic relation between the scanning photocurrent profile and the minority carrier decay length was established. Then the derived analytic formula was validated numerically and experimentally. This analytic formula provides a new fitting method for SPCM profiles to correctly determine the minority carrier decay length, which allows us to quantitatively evaluate the performance of nanowire-based devices.
format Online
Article
Text
id pubmed-6603194
institution National Center for Biotechnology Information
language English
publishDate 2019
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-66031942019-07-14 A New Analytic Formula for Minority Carrier Decay Length Extraction from Scanning Photocurrent Profiles in Ohmic-Contact Nanowire Devices Chu, Cheng-Hao Mao, Ming-Hua Yang, Che-Wei Lin, Hao-Hsiung Sci Rep Article Spatially resolved current measurements such as scanning photocurrent microscopy (SPCM) have been extensively applied to investigate carrier transport properties in semiconductor nanowires. A traditional simple-exponential-decay formula based on the assumption of carrier diffusion dominance in the scanning photocurrent profiles can be applied for carrier diffusion length extraction using SPCM in Schottky-contact-based or p-n junction-based devices where large built-in electric fields exist. However, it is also important to study the electric-field dependent transport properties in widely used ohmic-contact nanowire devices where the assumption of carrier diffusion dominance is invalid. Here we derive an analytic formula for scanning photocurrent profiles in such ohmic-contact nanowire devices under uniform applied electric fields and weak optical excitation. Under these operation conditions and the influence of photo-carrier-induced electric field, the scanning photocurrent profile and the carrier spatial distribution strikingly do not share the same functional form. Instead, a surprising new analytic relation between the scanning photocurrent profile and the minority carrier decay length was established. Then the derived analytic formula was validated numerically and experimentally. This analytic formula provides a new fitting method for SPCM profiles to correctly determine the minority carrier decay length, which allows us to quantitatively evaluate the performance of nanowire-based devices. Nature Publishing Group UK 2019-07-01 /pmc/articles/PMC6603194/ /pubmed/31263209 http://dx.doi.org/10.1038/s41598-019-46020-2 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Chu, Cheng-Hao
Mao, Ming-Hua
Yang, Che-Wei
Lin, Hao-Hsiung
A New Analytic Formula for Minority Carrier Decay Length Extraction from Scanning Photocurrent Profiles in Ohmic-Contact Nanowire Devices
title A New Analytic Formula for Minority Carrier Decay Length Extraction from Scanning Photocurrent Profiles in Ohmic-Contact Nanowire Devices
title_full A New Analytic Formula for Minority Carrier Decay Length Extraction from Scanning Photocurrent Profiles in Ohmic-Contact Nanowire Devices
title_fullStr A New Analytic Formula for Minority Carrier Decay Length Extraction from Scanning Photocurrent Profiles in Ohmic-Contact Nanowire Devices
title_full_unstemmed A New Analytic Formula for Minority Carrier Decay Length Extraction from Scanning Photocurrent Profiles in Ohmic-Contact Nanowire Devices
title_short A New Analytic Formula for Minority Carrier Decay Length Extraction from Scanning Photocurrent Profiles in Ohmic-Contact Nanowire Devices
title_sort new analytic formula for minority carrier decay length extraction from scanning photocurrent profiles in ohmic-contact nanowire devices
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6603194/
https://www.ncbi.nlm.nih.gov/pubmed/31263209
http://dx.doi.org/10.1038/s41598-019-46020-2
work_keys_str_mv AT chuchenghao anewanalyticformulaforminoritycarrierdecaylengthextractionfromscanningphotocurrentprofilesinohmiccontactnanowiredevices
AT maominghua anewanalyticformulaforminoritycarrierdecaylengthextractionfromscanningphotocurrentprofilesinohmiccontactnanowiredevices
AT yangchewei anewanalyticformulaforminoritycarrierdecaylengthextractionfromscanningphotocurrentprofilesinohmiccontactnanowiredevices
AT linhaohsiung anewanalyticformulaforminoritycarrierdecaylengthextractionfromscanningphotocurrentprofilesinohmiccontactnanowiredevices
AT chuchenghao newanalyticformulaforminoritycarrierdecaylengthextractionfromscanningphotocurrentprofilesinohmiccontactnanowiredevices
AT maominghua newanalyticformulaforminoritycarrierdecaylengthextractionfromscanningphotocurrentprofilesinohmiccontactnanowiredevices
AT yangchewei newanalyticformulaforminoritycarrierdecaylengthextractionfromscanningphotocurrentprofilesinohmiccontactnanowiredevices
AT linhaohsiung newanalyticformulaforminoritycarrierdecaylengthextractionfromscanningphotocurrentprofilesinohmiccontactnanowiredevices