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Vibrational Relaxation Dynamics of the Core and Outer Part of Proton-Hydration Clusters

[Image: see text] We study the ultrafast relaxation dynamics of hydrated proton clusters in acetonitrile using femtosecond mid-infrared pump-probe spectroscopy. We observe a strong dependence of transient absorption dynamics on the frequency of excitation. When we excite the OH vibrations with frequ...

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Detalles Bibliográficos
Autores principales: Sofronov, Oleksandr O., Bakker, Huib J.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2019
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6661761/
https://www.ncbi.nlm.nih.gov/pubmed/31265298
http://dx.doi.org/10.1021/acs.jpcb.9b02067