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Surface enhanced dynamic nuclear polarization solid-state NMR spectroscopy sheds light on Brønsted–Lewis acid synergy during the zeolite catalyzed methanol-to-hydrocarbon process

After a prolonged effort over two decades, the reaction mechanism of the zeolite-catalyzed methanol-to-hydrocarbon (MTH) process is now well-understood: the so-called ‘direct mechanism’ (via direct coupling of two methanol molecules) is responsible for the formation of the initial carbon–carbon bond...

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Detalles Bibliográficos
Autores principales: Dutta Chowdhury, Abhishek, Yarulina, Irina, Abou-Hamad, Edy, Gurinov, Andrei, Gascon, Jorge
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Royal Society of Chemistry 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7068724/
https://www.ncbi.nlm.nih.gov/pubmed/32190235
http://dx.doi.org/10.1039/c9sc02215e