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Polaritonic molecular clock for all-optical ultrafast imaging of wavepacket dynamics without probe pulses

Conventional approaches to probing ultrafast molecular dynamics rely on the use of synchronized laser pulses with a well-defined time delay. Typically, a pump pulse excites a molecular wavepacket. A subsequent probe pulse can then dissociate or ionize the molecule, and measurement of the molecular f...

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Detalles Bibliográficos
Autores principales: Silva, R. E. F., Pino, Javier del, García-Vidal, Francisco J., Feist, Johannes
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7078293/
https://www.ncbi.nlm.nih.gov/pubmed/32184408
http://dx.doi.org/10.1038/s41467-020-15196-x