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Fluctuating Storage of the Active Phase in a Mn‐Na(2)WO(4)/SiO(2) Catalyst for the Oxidative Coupling of Methane
Structural dynamics of a Mn‐Na(2)WO(4)/SiO(2) catalyst were detected directly under reaction conditions during the oxidative coupling of methane via in situ XRD and operando Raman spectroscopy. A new concept of fluctuating storage and release of an active phase in heterogeneous catalysis is proposed...
Autores principales: | , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
John Wiley and Sons Inc.
2020
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7496389/ https://www.ncbi.nlm.nih.gov/pubmed/32364281 http://dx.doi.org/10.1002/anie.202004778 |