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Surface Charges at the CaF(2)/Water Interface Allow Very Fast Intermolecular Vibrational‐Energy Transfer
We investigate the dynamics of water in contact with solid calcium fluoride, where at low pH, localized charges can develop upon fluorite dissolution. We use 2D surface‐specific vibrational spectroscopy to quantify the heterogeneity of the interfacial water (D(2)O) molecules and provide information...
Autores principales: | Lesnicki, Dominika, Zhang, Zhen, Bonn, Mischa, Sulpizi, Marialore, Backus, Ellen H. G. |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
John Wiley and Sons Inc.
2020
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7496624/ https://www.ncbi.nlm.nih.gov/pubmed/32239715 http://dx.doi.org/10.1002/anie.202004686 |
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