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Reorientation-induced relaxation of free OH at the air/water interface revealed by ultrafast heterodyne-detected nonlinear spectroscopy

The uniqueness of water originates from its three-dimensional hydrogen-bond network, but this hydrogen-bond network is suddenly truncated at the interface and non-hydrogen-bonded OH (free OH) appears. Although this free OH is the most characteristic feature of interfacial water, the molecular-level...

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Detalles Bibliográficos
Autores principales: Inoue, Ken-ichi, Ahmed, Mohammed, Nihonyanagi, Satoshi, Tahara, Tahei
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7581742/
https://www.ncbi.nlm.nih.gov/pubmed/33093482
http://dx.doi.org/10.1038/s41467-020-19143-8