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The Smoluchowski Ensemble—Statistical Mechanics of Aggregation
We present a rigorous thermodynamic treatment of irreversible binary aggregation. We construct the Smoluchowski ensemble as the set of discrete finite distributions that are reached in fixed number of merging events and define a probability measure on this ensemble, such that the mean distribution i...
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Formato: | Online Artículo Texto |
Lenguaje: | English |
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MDPI
2020
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7597352/ https://www.ncbi.nlm.nih.gov/pubmed/33286949 http://dx.doi.org/10.3390/e22101181 |