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Ion tracks in silicon formed by much lower energy deposition than the track formation threshold

Damaged regions of cylindrical shapes called ion tracks, typically in nano-meters wide and tens micro-meters long, are formed along the ion trajectories in many insulators, when high energy ions in the electronic stopping regime are injected. In most cases, the ion tracks were assumed as consequence...

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Autores principales: Amekura, H., Toulemonde, M., Narumi, K., Li, R., Chiba, A., Hirano, Y., Yamada, K., Yamamoto, S., Ishikawa, N., Okubo, N., Saitoh, Y.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7794553/
https://www.ncbi.nlm.nih.gov/pubmed/33420182
http://dx.doi.org/10.1038/s41598-020-80360-8
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author Amekura, H.
Toulemonde, M.
Narumi, K.
Li, R.
Chiba, A.
Hirano, Y.
Yamada, K.
Yamamoto, S.
Ishikawa, N.
Okubo, N.
Saitoh, Y.
author_facet Amekura, H.
Toulemonde, M.
Narumi, K.
Li, R.
Chiba, A.
Hirano, Y.
Yamada, K.
Yamamoto, S.
Ishikawa, N.
Okubo, N.
Saitoh, Y.
author_sort Amekura, H.
collection PubMed
description Damaged regions of cylindrical shapes called ion tracks, typically in nano-meters wide and tens micro-meters long, are formed along the ion trajectories in many insulators, when high energy ions in the electronic stopping regime are injected. In most cases, the ion tracks were assumed as consequences of dense electronic energy deposition from the high energy ions, except some cases where the synergy effect with the nuclear energy deposition plays an important role. In crystalline Si (c-Si), no tracks have been observed with any monomer ions up to GeV. Tracks are formed in c-Si under 40 MeV fullerene (C(60)) cluster ion irradiation, which provides much higher energy deposition than monomer ions. The track diameter decreases with decreasing the ion energy until they disappear at an extrapolated value of ~ 17 MeV. However, here we report the track formation of 10 nm in diameter under C(60) ion irradiation of 6 MeV, i.e., much lower than the extrapolated threshold. The diameters of 10 nm were comparable to those under 40 MeV C(60) irradiation. Furthermore, the tracks formed by 6 MeV C(60) irradiation consisted of damaged crystalline, while those formed by 40 MeV C(60) irradiation were amorphous. The track formation was observed down to 1 MeV and probably lower with decreasing the track diameters. The track lengths were much shorter than those expected from the drop of S(e) below the threshold. These track formations at such low energies cannot be explained by the conventional purely electronic energy deposition mechanism, indicating another origin, e.g., the synergy effect between the electronic and nuclear energy depositions, or dual transitions of transient melting and boiling.
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spelling pubmed-77945532021-01-12 Ion tracks in silicon formed by much lower energy deposition than the track formation threshold Amekura, H. Toulemonde, M. Narumi, K. Li, R. Chiba, A. Hirano, Y. Yamada, K. Yamamoto, S. Ishikawa, N. Okubo, N. Saitoh, Y. Sci Rep Article Damaged regions of cylindrical shapes called ion tracks, typically in nano-meters wide and tens micro-meters long, are formed along the ion trajectories in many insulators, when high energy ions in the electronic stopping regime are injected. In most cases, the ion tracks were assumed as consequences of dense electronic energy deposition from the high energy ions, except some cases where the synergy effect with the nuclear energy deposition plays an important role. In crystalline Si (c-Si), no tracks have been observed with any monomer ions up to GeV. Tracks are formed in c-Si under 40 MeV fullerene (C(60)) cluster ion irradiation, which provides much higher energy deposition than monomer ions. The track diameter decreases with decreasing the ion energy until they disappear at an extrapolated value of ~ 17 MeV. However, here we report the track formation of 10 nm in diameter under C(60) ion irradiation of 6 MeV, i.e., much lower than the extrapolated threshold. The diameters of 10 nm were comparable to those under 40 MeV C(60) irradiation. Furthermore, the tracks formed by 6 MeV C(60) irradiation consisted of damaged crystalline, while those formed by 40 MeV C(60) irradiation were amorphous. The track formation was observed down to 1 MeV and probably lower with decreasing the track diameters. The track lengths were much shorter than those expected from the drop of S(e) below the threshold. These track formations at such low energies cannot be explained by the conventional purely electronic energy deposition mechanism, indicating another origin, e.g., the synergy effect between the electronic and nuclear energy depositions, or dual transitions of transient melting and boiling. Nature Publishing Group UK 2021-01-08 /pmc/articles/PMC7794553/ /pubmed/33420182 http://dx.doi.org/10.1038/s41598-020-80360-8 Text en © The Author(s) 2021 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Amekura, H.
Toulemonde, M.
Narumi, K.
Li, R.
Chiba, A.
Hirano, Y.
Yamada, K.
Yamamoto, S.
Ishikawa, N.
Okubo, N.
Saitoh, Y.
Ion tracks in silicon formed by much lower energy deposition than the track formation threshold
title Ion tracks in silicon formed by much lower energy deposition than the track formation threshold
title_full Ion tracks in silicon formed by much lower energy deposition than the track formation threshold
title_fullStr Ion tracks in silicon formed by much lower energy deposition than the track formation threshold
title_full_unstemmed Ion tracks in silicon formed by much lower energy deposition than the track formation threshold
title_short Ion tracks in silicon formed by much lower energy deposition than the track formation threshold
title_sort ion tracks in silicon formed by much lower energy deposition than the track formation threshold
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7794553/
https://www.ncbi.nlm.nih.gov/pubmed/33420182
http://dx.doi.org/10.1038/s41598-020-80360-8
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