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Light Emission in Metal–Semiconductor Tunnel Junctions: Direct Evidence for Electron Heating by Plasmon Decay

[Image: see text] We study metal–insulator–semiconductor tunnel junctions where the metal electrode is a patterned gold layer, the insulator is a thin layer of Al(2)O(3), and the semiconductor is p-type silicon. We observe light emission due to plasmon-assisted inelastic tunneling from the metal to...

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Autores principales: Shalem, Guy, Erez-Cohen, Omer, Mahalu, Diana, Bar-Joseph, Israel
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7883388/
https://www.ncbi.nlm.nih.gov/pubmed/33497237
http://dx.doi.org/10.1021/acs.nanolett.0c03945
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author Shalem, Guy
Erez-Cohen, Omer
Mahalu, Diana
Bar-Joseph, Israel
author_facet Shalem, Guy
Erez-Cohen, Omer
Mahalu, Diana
Bar-Joseph, Israel
author_sort Shalem, Guy
collection PubMed
description [Image: see text] We study metal–insulator–semiconductor tunnel junctions where the metal electrode is a patterned gold layer, the insulator is a thin layer of Al(2)O(3), and the semiconductor is p-type silicon. We observe light emission due to plasmon-assisted inelastic tunneling from the metal to the silicon valence band. The emission cutoff shifts to higher energies with increasing voltage, a clear signature of electrically driven plasmons. The cutoff energy exceeds the applied voltage, and a large fraction of the emission is above the threshold, ℏω > eV. We find that the emission spectrum manifests the Fermi–Dirac distribution of the electrons in the gold electrode. This distribution can be used to determine the effective electron temperature, T(e), which is shown to have a linear dependence on the applied voltage. The strong correlation of T(e) with the plasmon energy serves as evidence that the mechanism for heating the electrons is plasmon decay at the source metal electrode.
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spelling pubmed-78833882021-02-16 Light Emission in Metal–Semiconductor Tunnel Junctions: Direct Evidence for Electron Heating by Plasmon Decay Shalem, Guy Erez-Cohen, Omer Mahalu, Diana Bar-Joseph, Israel Nano Lett [Image: see text] We study metal–insulator–semiconductor tunnel junctions where the metal electrode is a patterned gold layer, the insulator is a thin layer of Al(2)O(3), and the semiconductor is p-type silicon. We observe light emission due to plasmon-assisted inelastic tunneling from the metal to the silicon valence band. The emission cutoff shifts to higher energies with increasing voltage, a clear signature of electrically driven plasmons. The cutoff energy exceeds the applied voltage, and a large fraction of the emission is above the threshold, ℏω > eV. We find that the emission spectrum manifests the Fermi–Dirac distribution of the electrons in the gold electrode. This distribution can be used to determine the effective electron temperature, T(e), which is shown to have a linear dependence on the applied voltage. The strong correlation of T(e) with the plasmon energy serves as evidence that the mechanism for heating the electrons is plasmon decay at the source metal electrode. American Chemical Society 2021-01-26 2021-02-10 /pmc/articles/PMC7883388/ /pubmed/33497237 http://dx.doi.org/10.1021/acs.nanolett.0c03945 Text en © 2021 American Chemical Society This is an open access article published under a Creative Commons Attribution (CC-BY) License (http://pubs.acs.org/page/policy/authorchoice_ccby_termsofuse.html) , which permits unrestricted use, distribution and reproduction in any medium, provided the author and source are cited.
spellingShingle Shalem, Guy
Erez-Cohen, Omer
Mahalu, Diana
Bar-Joseph, Israel
Light Emission in Metal–Semiconductor Tunnel Junctions: Direct Evidence for Electron Heating by Plasmon Decay
title Light Emission in Metal–Semiconductor Tunnel Junctions: Direct Evidence for Electron Heating by Plasmon Decay
title_full Light Emission in Metal–Semiconductor Tunnel Junctions: Direct Evidence for Electron Heating by Plasmon Decay
title_fullStr Light Emission in Metal–Semiconductor Tunnel Junctions: Direct Evidence for Electron Heating by Plasmon Decay
title_full_unstemmed Light Emission in Metal–Semiconductor Tunnel Junctions: Direct Evidence for Electron Heating by Plasmon Decay
title_short Light Emission in Metal–Semiconductor Tunnel Junctions: Direct Evidence for Electron Heating by Plasmon Decay
title_sort light emission in metal–semiconductor tunnel junctions: direct evidence for electron heating by plasmon decay
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7883388/
https://www.ncbi.nlm.nih.gov/pubmed/33497237
http://dx.doi.org/10.1021/acs.nanolett.0c03945
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