Cargando…
Light Emission in Metal–Semiconductor Tunnel Junctions: Direct Evidence for Electron Heating by Plasmon Decay
[Image: see text] We study metal–insulator–semiconductor tunnel junctions where the metal electrode is a patterned gold layer, the insulator is a thin layer of Al(2)O(3), and the semiconductor is p-type silicon. We observe light emission due to plasmon-assisted inelastic tunneling from the metal to...
Autores principales: | , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2021
|
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7883388/ https://www.ncbi.nlm.nih.gov/pubmed/33497237 http://dx.doi.org/10.1021/acs.nanolett.0c03945 |
_version_ | 1783651202541551616 |
---|---|
author | Shalem, Guy Erez-Cohen, Omer Mahalu, Diana Bar-Joseph, Israel |
author_facet | Shalem, Guy Erez-Cohen, Omer Mahalu, Diana Bar-Joseph, Israel |
author_sort | Shalem, Guy |
collection | PubMed |
description | [Image: see text] We study metal–insulator–semiconductor tunnel junctions where the metal electrode is a patterned gold layer, the insulator is a thin layer of Al(2)O(3), and the semiconductor is p-type silicon. We observe light emission due to plasmon-assisted inelastic tunneling from the metal to the silicon valence band. The emission cutoff shifts to higher energies with increasing voltage, a clear signature of electrically driven plasmons. The cutoff energy exceeds the applied voltage, and a large fraction of the emission is above the threshold, ℏω > eV. We find that the emission spectrum manifests the Fermi–Dirac distribution of the electrons in the gold electrode. This distribution can be used to determine the effective electron temperature, T(e), which is shown to have a linear dependence on the applied voltage. The strong correlation of T(e) with the plasmon energy serves as evidence that the mechanism for heating the electrons is plasmon decay at the source metal electrode. |
format | Online Article Text |
id | pubmed-7883388 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-78833882021-02-16 Light Emission in Metal–Semiconductor Tunnel Junctions: Direct Evidence for Electron Heating by Plasmon Decay Shalem, Guy Erez-Cohen, Omer Mahalu, Diana Bar-Joseph, Israel Nano Lett [Image: see text] We study metal–insulator–semiconductor tunnel junctions where the metal electrode is a patterned gold layer, the insulator is a thin layer of Al(2)O(3), and the semiconductor is p-type silicon. We observe light emission due to plasmon-assisted inelastic tunneling from the metal to the silicon valence band. The emission cutoff shifts to higher energies with increasing voltage, a clear signature of electrically driven plasmons. The cutoff energy exceeds the applied voltage, and a large fraction of the emission is above the threshold, ℏω > eV. We find that the emission spectrum manifests the Fermi–Dirac distribution of the electrons in the gold electrode. This distribution can be used to determine the effective electron temperature, T(e), which is shown to have a linear dependence on the applied voltage. The strong correlation of T(e) with the plasmon energy serves as evidence that the mechanism for heating the electrons is plasmon decay at the source metal electrode. American Chemical Society 2021-01-26 2021-02-10 /pmc/articles/PMC7883388/ /pubmed/33497237 http://dx.doi.org/10.1021/acs.nanolett.0c03945 Text en © 2021 American Chemical Society This is an open access article published under a Creative Commons Attribution (CC-BY) License (http://pubs.acs.org/page/policy/authorchoice_ccby_termsofuse.html) , which permits unrestricted use, distribution and reproduction in any medium, provided the author and source are cited. |
spellingShingle | Shalem, Guy Erez-Cohen, Omer Mahalu, Diana Bar-Joseph, Israel Light Emission in Metal–Semiconductor Tunnel Junctions: Direct Evidence for Electron Heating by Plasmon Decay |
title | Light Emission in Metal–Semiconductor Tunnel
Junctions: Direct Evidence for Electron Heating by Plasmon Decay |
title_full | Light Emission in Metal–Semiconductor Tunnel
Junctions: Direct Evidence for Electron Heating by Plasmon Decay |
title_fullStr | Light Emission in Metal–Semiconductor Tunnel
Junctions: Direct Evidence for Electron Heating by Plasmon Decay |
title_full_unstemmed | Light Emission in Metal–Semiconductor Tunnel
Junctions: Direct Evidence for Electron Heating by Plasmon Decay |
title_short | Light Emission in Metal–Semiconductor Tunnel
Junctions: Direct Evidence for Electron Heating by Plasmon Decay |
title_sort | light emission in metal–semiconductor tunnel
junctions: direct evidence for electron heating by plasmon decay |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7883388/ https://www.ncbi.nlm.nih.gov/pubmed/33497237 http://dx.doi.org/10.1021/acs.nanolett.0c03945 |
work_keys_str_mv | AT shalemguy lightemissioninmetalsemiconductortunneljunctionsdirectevidenceforelectronheatingbyplasmondecay AT erezcohenomer lightemissioninmetalsemiconductortunneljunctionsdirectevidenceforelectronheatingbyplasmondecay AT mahaludiana lightemissioninmetalsemiconductortunneljunctionsdirectevidenceforelectronheatingbyplasmondecay AT barjosephisrael lightemissioninmetalsemiconductortunneljunctionsdirectevidenceforelectronheatingbyplasmondecay |