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Wet-Etched Microlens Array for 200 nm Spatial Isolation of Epitaxial Single QDs and 80 nm Broadband Enhancement of Their Quantum Light Extraction

Uniform arrays of three shapes ([Formula: see text] , [Formula: see text] , and [Formula: see text]) of GaAs microlenses (MLs) by wet-etching are demonstrated, ∼200 nm spatial isolation of epitaxial single QDs embedded ([Formula: see text]: 890–990 nm) and broadband ([Formula: see text] nm) enhancem...

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Autores principales: Li, Shulun, Shang, Xiangjun, Chen, Yao, Su, Xiangbin, Hao, Huiming, Liu, Hanqing, Zhang, Yu, Ni, Haiqiao, Niu, Zhichuan
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8146877/
https://www.ncbi.nlm.nih.gov/pubmed/33925761
http://dx.doi.org/10.3390/nano11051136
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author Li, Shulun
Shang, Xiangjun
Chen, Yao
Su, Xiangbin
Hao, Huiming
Liu, Hanqing
Zhang, Yu
Ni, Haiqiao
Niu, Zhichuan
author_facet Li, Shulun
Shang, Xiangjun
Chen, Yao
Su, Xiangbin
Hao, Huiming
Liu, Hanqing
Zhang, Yu
Ni, Haiqiao
Niu, Zhichuan
author_sort Li, Shulun
collection PubMed
description Uniform arrays of three shapes ([Formula: see text] , [Formula: see text] , and [Formula: see text]) of GaAs microlenses (MLs) by wet-etching are demonstrated, ∼200 nm spatial isolation of epitaxial single QDs embedded ([Formula: see text]: 890–990 nm) and broadband ([Formula: see text] nm) enhancement of their quantum light extraction are obtained, which is also suitable for telecom-band epitaxial QDs. Combined with the bottom distributed Bragg reflector, the [Formula: see text]-shaped ML forms a cavity and achieves the best enhancement: extraction efficiency of 26%, Purcell factor of 2 and single-photon count rate of [Formula: see text] counts per second at the first lens; while the [Formula: see text]-shaped ML shows a broader band (e.g., longer [Formula: see text]) enhancement. In the MLs, single QDs with featured exciton emissions are observed, whose time correlations prove single-photon emission with multi-photon probability [Formula: see text]; some QDs show both biexciton [Formula: see text] and exciton X emissions and exhibit a perfect cascade feature. This work could pave a step towards a scalable array of QD single-photon sources and the application of QD photon-pair emission for entanglement experiments.
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spelling pubmed-81468772021-05-26 Wet-Etched Microlens Array for 200 nm Spatial Isolation of Epitaxial Single QDs and 80 nm Broadband Enhancement of Their Quantum Light Extraction Li, Shulun Shang, Xiangjun Chen, Yao Su, Xiangbin Hao, Huiming Liu, Hanqing Zhang, Yu Ni, Haiqiao Niu, Zhichuan Nanomaterials (Basel) Article Uniform arrays of three shapes ([Formula: see text] , [Formula: see text] , and [Formula: see text]) of GaAs microlenses (MLs) by wet-etching are demonstrated, ∼200 nm spatial isolation of epitaxial single QDs embedded ([Formula: see text]: 890–990 nm) and broadband ([Formula: see text] nm) enhancement of their quantum light extraction are obtained, which is also suitable for telecom-band epitaxial QDs. Combined with the bottom distributed Bragg reflector, the [Formula: see text]-shaped ML forms a cavity and achieves the best enhancement: extraction efficiency of 26%, Purcell factor of 2 and single-photon count rate of [Formula: see text] counts per second at the first lens; while the [Formula: see text]-shaped ML shows a broader band (e.g., longer [Formula: see text]) enhancement. In the MLs, single QDs with featured exciton emissions are observed, whose time correlations prove single-photon emission with multi-photon probability [Formula: see text]; some QDs show both biexciton [Formula: see text] and exciton X emissions and exhibit a perfect cascade feature. This work could pave a step towards a scalable array of QD single-photon sources and the application of QD photon-pair emission for entanglement experiments. MDPI 2021-04-27 /pmc/articles/PMC8146877/ /pubmed/33925761 http://dx.doi.org/10.3390/nano11051136 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Li, Shulun
Shang, Xiangjun
Chen, Yao
Su, Xiangbin
Hao, Huiming
Liu, Hanqing
Zhang, Yu
Ni, Haiqiao
Niu, Zhichuan
Wet-Etched Microlens Array for 200 nm Spatial Isolation of Epitaxial Single QDs and 80 nm Broadband Enhancement of Their Quantum Light Extraction
title Wet-Etched Microlens Array for 200 nm Spatial Isolation of Epitaxial Single QDs and 80 nm Broadband Enhancement of Their Quantum Light Extraction
title_full Wet-Etched Microlens Array for 200 nm Spatial Isolation of Epitaxial Single QDs and 80 nm Broadband Enhancement of Their Quantum Light Extraction
title_fullStr Wet-Etched Microlens Array for 200 nm Spatial Isolation of Epitaxial Single QDs and 80 nm Broadband Enhancement of Their Quantum Light Extraction
title_full_unstemmed Wet-Etched Microlens Array for 200 nm Spatial Isolation of Epitaxial Single QDs and 80 nm Broadband Enhancement of Their Quantum Light Extraction
title_short Wet-Etched Microlens Array for 200 nm Spatial Isolation of Epitaxial Single QDs and 80 nm Broadband Enhancement of Their Quantum Light Extraction
title_sort wet-etched microlens array for 200 nm spatial isolation of epitaxial single qds and 80 nm broadband enhancement of their quantum light extraction
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8146877/
https://www.ncbi.nlm.nih.gov/pubmed/33925761
http://dx.doi.org/10.3390/nano11051136
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