Cargando…

Observation of Electric-Field-Induced Structural Dislocations in a Ferroelectric Oxide

[Image: see text] Dislocations are 1D topological defects with emergent electronic properties. Their low dimensionality and unique properties make them excellent candidates for innovative device concepts, ranging from dislocation-based neuromorphic memory to light emission from diodes. To date, disl...

Descripción completa

Detalles Bibliográficos
Autores principales: Evans, Donald M., Småbråten, Didrik René, Holstad, Theodor S., Vullum, Per Erik, Mosberg, Aleksander B., Yan, Zewu, Bourret, Edith, van Helvoort, Antonius T. J., Selbach, Sverre M., Meier, Dennis
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8155316/
https://www.ncbi.nlm.nih.gov/pubmed/33861614
http://dx.doi.org/10.1021/acs.nanolett.0c04816
_version_ 1783699174541230080
author Evans, Donald M.
Småbråten, Didrik René
Holstad, Theodor S.
Vullum, Per Erik
Mosberg, Aleksander B.
Yan, Zewu
Bourret, Edith
van Helvoort, Antonius T. J.
Selbach, Sverre M.
Meier, Dennis
author_facet Evans, Donald M.
Småbråten, Didrik René
Holstad, Theodor S.
Vullum, Per Erik
Mosberg, Aleksander B.
Yan, Zewu
Bourret, Edith
van Helvoort, Antonius T. J.
Selbach, Sverre M.
Meier, Dennis
author_sort Evans, Donald M.
collection PubMed
description [Image: see text] Dislocations are 1D topological defects with emergent electronic properties. Their low dimensionality and unique properties make them excellent candidates for innovative device concepts, ranging from dislocation-based neuromorphic memory to light emission from diodes. To date, dislocations are created in materials during synthesis via strain fields or flash sintering or retrospectively via deformation, for example, (nano)-indentation, limiting the technological possibilities. In this work, we demonstrate the creation of dislocations in the ferroelectric semiconductor Er(Mn,Ti)O(3) with nanoscale spatial precision using electric fields. By combining high-resolution imaging techniques and density functional theory calculations, direct images of the dislocations are collected, and their impact on the local electric transport behavior is studied. Our approach enables local property control via dislocations without the need for external macroscopic strain fields, expanding the application opportunities into the realm of electric-field-driven phenomena.
format Online
Article
Text
id pubmed-8155316
institution National Center for Biotechnology Information
language English
publishDate 2021
publisher American Chemical Society
record_format MEDLINE/PubMed
spelling pubmed-81553162021-05-28 Observation of Electric-Field-Induced Structural Dislocations in a Ferroelectric Oxide Evans, Donald M. Småbråten, Didrik René Holstad, Theodor S. Vullum, Per Erik Mosberg, Aleksander B. Yan, Zewu Bourret, Edith van Helvoort, Antonius T. J. Selbach, Sverre M. Meier, Dennis Nano Lett [Image: see text] Dislocations are 1D topological defects with emergent electronic properties. Their low dimensionality and unique properties make them excellent candidates for innovative device concepts, ranging from dislocation-based neuromorphic memory to light emission from diodes. To date, dislocations are created in materials during synthesis via strain fields or flash sintering or retrospectively via deformation, for example, (nano)-indentation, limiting the technological possibilities. In this work, we demonstrate the creation of dislocations in the ferroelectric semiconductor Er(Mn,Ti)O(3) with nanoscale spatial precision using electric fields. By combining high-resolution imaging techniques and density functional theory calculations, direct images of the dislocations are collected, and their impact on the local electric transport behavior is studied. Our approach enables local property control via dislocations without the need for external macroscopic strain fields, expanding the application opportunities into the realm of electric-field-driven phenomena. American Chemical Society 2021-04-16 2021-04-28 /pmc/articles/PMC8155316/ /pubmed/33861614 http://dx.doi.org/10.1021/acs.nanolett.0c04816 Text en © 2021 The Authors. Published by American Chemical Society Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Evans, Donald M.
Småbråten, Didrik René
Holstad, Theodor S.
Vullum, Per Erik
Mosberg, Aleksander B.
Yan, Zewu
Bourret, Edith
van Helvoort, Antonius T. J.
Selbach, Sverre M.
Meier, Dennis
Observation of Electric-Field-Induced Structural Dislocations in a Ferroelectric Oxide
title Observation of Electric-Field-Induced Structural Dislocations in a Ferroelectric Oxide
title_full Observation of Electric-Field-Induced Structural Dislocations in a Ferroelectric Oxide
title_fullStr Observation of Electric-Field-Induced Structural Dislocations in a Ferroelectric Oxide
title_full_unstemmed Observation of Electric-Field-Induced Structural Dislocations in a Ferroelectric Oxide
title_short Observation of Electric-Field-Induced Structural Dislocations in a Ferroelectric Oxide
title_sort observation of electric-field-induced structural dislocations in a ferroelectric oxide
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8155316/
https://www.ncbi.nlm.nih.gov/pubmed/33861614
http://dx.doi.org/10.1021/acs.nanolett.0c04816
work_keys_str_mv AT evansdonaldm observationofelectricfieldinducedstructuraldislocationsinaferroelectricoxide
AT smabratendidrikrene observationofelectricfieldinducedstructuraldislocationsinaferroelectricoxide
AT holstadtheodors observationofelectricfieldinducedstructuraldislocationsinaferroelectricoxide
AT vullumpererik observationofelectricfieldinducedstructuraldislocationsinaferroelectricoxide
AT mosbergaleksanderb observationofelectricfieldinducedstructuraldislocationsinaferroelectricoxide
AT yanzewu observationofelectricfieldinducedstructuraldislocationsinaferroelectricoxide
AT bourretedith observationofelectricfieldinducedstructuraldislocationsinaferroelectricoxide
AT vanhelvoortantoniustj observationofelectricfieldinducedstructuraldislocationsinaferroelectricoxide
AT selbachsverrem observationofelectricfieldinducedstructuraldislocationsinaferroelectricoxide
AT meierdennis observationofelectricfieldinducedstructuraldislocationsinaferroelectricoxide