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Observation of Electric-Field-Induced Structural Dislocations in a Ferroelectric Oxide
[Image: see text] Dislocations are 1D topological defects with emergent electronic properties. Their low dimensionality and unique properties make them excellent candidates for innovative device concepts, ranging from dislocation-based neuromorphic memory to light emission from diodes. To date, disl...
Autores principales: | , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American
Chemical Society
2021
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8155316/ https://www.ncbi.nlm.nih.gov/pubmed/33861614 http://dx.doi.org/10.1021/acs.nanolett.0c04816 |
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author | Evans, Donald M. Småbråten, Didrik René Holstad, Theodor S. Vullum, Per Erik Mosberg, Aleksander B. Yan, Zewu Bourret, Edith van Helvoort, Antonius T. J. Selbach, Sverre M. Meier, Dennis |
author_facet | Evans, Donald M. Småbråten, Didrik René Holstad, Theodor S. Vullum, Per Erik Mosberg, Aleksander B. Yan, Zewu Bourret, Edith van Helvoort, Antonius T. J. Selbach, Sverre M. Meier, Dennis |
author_sort | Evans, Donald M. |
collection | PubMed |
description | [Image: see text] Dislocations are 1D topological defects with emergent electronic properties. Their low dimensionality and unique properties make them excellent candidates for innovative device concepts, ranging from dislocation-based neuromorphic memory to light emission from diodes. To date, dislocations are created in materials during synthesis via strain fields or flash sintering or retrospectively via deformation, for example, (nano)-indentation, limiting the technological possibilities. In this work, we demonstrate the creation of dislocations in the ferroelectric semiconductor Er(Mn,Ti)O(3) with nanoscale spatial precision using electric fields. By combining high-resolution imaging techniques and density functional theory calculations, direct images of the dislocations are collected, and their impact on the local electric transport behavior is studied. Our approach enables local property control via dislocations without the need for external macroscopic strain fields, expanding the application opportunities into the realm of electric-field-driven phenomena. |
format | Online Article Text |
id | pubmed-8155316 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | American
Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-81553162021-05-28 Observation of Electric-Field-Induced Structural Dislocations in a Ferroelectric Oxide Evans, Donald M. Småbråten, Didrik René Holstad, Theodor S. Vullum, Per Erik Mosberg, Aleksander B. Yan, Zewu Bourret, Edith van Helvoort, Antonius T. J. Selbach, Sverre M. Meier, Dennis Nano Lett [Image: see text] Dislocations are 1D topological defects with emergent electronic properties. Their low dimensionality and unique properties make them excellent candidates for innovative device concepts, ranging from dislocation-based neuromorphic memory to light emission from diodes. To date, dislocations are created in materials during synthesis via strain fields or flash sintering or retrospectively via deformation, for example, (nano)-indentation, limiting the technological possibilities. In this work, we demonstrate the creation of dislocations in the ferroelectric semiconductor Er(Mn,Ti)O(3) with nanoscale spatial precision using electric fields. By combining high-resolution imaging techniques and density functional theory calculations, direct images of the dislocations are collected, and their impact on the local electric transport behavior is studied. Our approach enables local property control via dislocations without the need for external macroscopic strain fields, expanding the application opportunities into the realm of electric-field-driven phenomena. American Chemical Society 2021-04-16 2021-04-28 /pmc/articles/PMC8155316/ /pubmed/33861614 http://dx.doi.org/10.1021/acs.nanolett.0c04816 Text en © 2021 The Authors. Published by American Chemical Society Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Evans, Donald M. Småbråten, Didrik René Holstad, Theodor S. Vullum, Per Erik Mosberg, Aleksander B. Yan, Zewu Bourret, Edith van Helvoort, Antonius T. J. Selbach, Sverre M. Meier, Dennis Observation of Electric-Field-Induced Structural Dislocations in a Ferroelectric Oxide |
title | Observation of Electric-Field-Induced Structural Dislocations
in a Ferroelectric Oxide |
title_full | Observation of Electric-Field-Induced Structural Dislocations
in a Ferroelectric Oxide |
title_fullStr | Observation of Electric-Field-Induced Structural Dislocations
in a Ferroelectric Oxide |
title_full_unstemmed | Observation of Electric-Field-Induced Structural Dislocations
in a Ferroelectric Oxide |
title_short | Observation of Electric-Field-Induced Structural Dislocations
in a Ferroelectric Oxide |
title_sort | observation of electric-field-induced structural dislocations
in a ferroelectric oxide |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8155316/ https://www.ncbi.nlm.nih.gov/pubmed/33861614 http://dx.doi.org/10.1021/acs.nanolett.0c04816 |
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