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Broad-band spectroscopy of a vanadyl porphyrin: a model electronuclear spin qudit

We explore how to encode more than a qubit in vanadyl porphyrin molecules hosting a S = 1/2 electronic spin coupled to a I = 7/2 nuclear spin. The spin Hamiltonian and its parameters, as well as the spin dynamics, have been determined via a combination of electron paramagnetic resonance, heat capaci...

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Detalles Bibliográficos
Autores principales: Gimeno, Ignacio, Urtizberea, Ainhoa, Román-Roche, Juan, Zueco, David, Camón, Agustín, Alonso, Pablo J., Roubeau, Olivier, Luis, Fernando
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8179683/
https://www.ncbi.nlm.nih.gov/pubmed/34168797
http://dx.doi.org/10.1039/d1sc00564b