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Ion correlations drive charge overscreening and heterogeneous nucleation at solid–aqueous electrolyte interfaces
Classical electrical double layer (EDL) models are foundational to the representation of atomistic structure and reactivity at charged interfaces. An important limitation to these models is their dependence on a mean-field approximation that is strictly valid for dilute aqueous solutions. Theoretica...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
National Academy of Sciences
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8364158/ https://www.ncbi.nlm.nih.gov/pubmed/34353907 http://dx.doi.org/10.1073/pnas.2105154118 |