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Degradation and regeneration of Fe–N(x) active sites for the oxygen reduction reaction: the role of surface oxidation, Fe demetallation and local carbon microporosity

The severe degradation of Fe–N–C electrocatalysts during a long-term oxygen reduction reaction (ORR) has become a major obstacle for application in proton-exchange membrane fuel cells. Understanding the degradation mechanism and regeneration of aged Fe–N–C catalysts would be of particular interest f...

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Detalles Bibliográficos
Autores principales: Xia, Dongsheng, Yu, Chenchen, Zhao, Yinghao, Wei, Yinping, Wu, Haiyan, Kang, Yongqiang, Li, Jia, Gan, Lin, Kang, Feiyu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8409490/
https://www.ncbi.nlm.nih.gov/pubmed/34567505
http://dx.doi.org/10.1039/d1sc03754d